Theory of Optically-Driven Sideband Cooling for Atomic Collective Excitations and Its Generalization

Theory of Optically-Driven Sideband Cooling for Atomic Collective Excitations and Its Generalization


We explore how to cool atomic collective excitations in an optically-driven three-level atomic ensemble, which may be described by a model of coupled two harmonic oscillators (HOs) with a time-dependent coupling. Moreover, the coupled two-HO model is further generalized to address other cooling issues, where the lower-frequency HO can be cooled whenever the cooling process dominates over the heating one during the sideband transitions. Unusually, due to the absence of the heating process, the optimal cooling of our first cooling protocol for collective excitations in an atomic ensemble could break a usual sideband cooling limit for general coupled two-HO models.

03.65.-w, 37.10.De, 43.58.Wc

Introduction.- Recently, quantum information processing based on collective excitations in atomic ensembles has attracted more and more attentions. Photons are good carriers of quantum information due to their fast velocity and low leakage, while may not be easy to store. Naturally, it is desired to study atomic ensembles as potential quantum memory units of photons due to the long coherence time. Interestingly, the form-stable dark-state polariton (DSP) (1) associated with the propagation of quantum optical fields via electromagnetically induced transparency (EIT) (2), was proposed in a three-level -type atomic ensemble. In the low excitations limit, DSP can be described as a hybrid bosonic mode (3). By controlling the mixing angle between light and matter components of DSP, the optical pulse can be decelerated and “trapped” via mapping its shape and quantum state onto meta-stable collective-excitation state of matter. That means the quantum information storage (1); (3); (4) can be achieved in the atomic ensembles by adiabatically controlling the coupling.

As is known, collective excitations could also be used in quantum communication in atomic ensembles and linear optics. Since the work of Duan-Lukin-Cirac-Zoller (5), a number of protocols (6); (7); (8); (9) have been proposed to implement robust long-distance quantum communications, quantum repeaters, and quantum information storages based on atomic ensembles over long photonic lossy channels.

In a realistic atomic ensemble, a given collective-excitation mode may have a finite thermal population due to the interaction with the thermal bath at finite temperature. This means that it is necessary to cool the thermal excitations in quantum information processing based on atomic collective excitations. In this Letter, we consider a driven three-level atomic ensemble that can be modeled by coupled two harmonic resonators (HOs), and then elaborate how to cool the low-frequency collective-excitation mode near its ground state in this kind of systems.

On the other hand, various nano- (or submicron-) mechanical resonators have been investigated (10) extensively in recent years. To reveal the quantum effect in the nano-mechanical devices, various cooling schemes (11); (12); (13); (14); (15); (16) were proposed to drive them to reach the standard quantum limit (SQL) (17). A famous one among them is the optical radiation-pressure cooling scheme (12) attributed to the (resolved) sideband cooling (13); (14); (15); (16), which was previously well-developed to cool the spatial motion of the trapped ions (18) or the neutral atoms (19). Notably, our cooling scheme for atomic ensembles is based on the sideband structure induced by the lower-frequency mode, which is time-dependently coupled with the higher-frequency mode to loss its energy. Moreover, we generalize the above coupled two-HO model to other two types of cooling model beyond the optical radiation-pressure cooling of mechanical resonator. In the generalized model, the lower-frequency HO can be cooled with a usual sideband cooling limit, whose cooling mechanism can also be employed to understand the cooling of collective excitations in the atomic ensembles. It is remarkable that our protocol of atomic ensemble breaks the limit of usual sideband cooling due to the absence of counter-rotating terms in such a coupled two-HO model.

Three-Level atomic ensemble modeled by two coupled oscillators.- Let us consider an ensemble of identical three-level atoms as seen in Fig. 1(a). A strong classical driving light field is homogenously coupled to each atomic transition from the metastable state to the excited one . Then the Hamiltonian reads ( hereafter)


where are the corresponding energies of the atomic states , and respectively, and the ground state energy . is the coupling strength of the driving light field (with the carrier frequency ), which can be assumed to be real.

Figure 1: (Color online) (a) Three-level atomic ensemble with most atoms staying in the ground states . The strong driving light couples to the transition from the meta-stable state to the excited one for each atom. The electric-dipole transition is permitted, but is forbidden. The waved lines denote the decay processes with the corresponding decay rates. (b) The cooling process () and (c) the heating process () for mode starting form in the sideband structure forming by splitting a-mode with the low-frequency b-mode. ( and ( are the detunings for the anti-Stokes (cooling) and Stokes (heating) transitions, respectively.

Normally, a weak quantized probe light would couple to the transition . Thus, a so-called -type three-level atomic ensemble configuration can be constructed associated with the well-known EIT and group-velocity slowdown phenomena. In such an ensemble, the DSP can also be obtained as the superposition of the optical mode and the atomic collective-excitation mode (1); (3); (4). Based on the notations of EIT and DSP, the atomic ensemble can be a unit of quantum memory and be used to store the quantum information of, e.g., the photons. Here, we focus only on the cooling of the atomic collective excitations in the absence of the probe light field, also noting that extensive studies have been made in the framework of optically-pumping an individual atom into its internal lowest-energy ground state (20).

We now introduce the bosonic operators and for atomic collective excitations (3); (21), which satisfy , and in the limit of with low excitations. Then, Hamiltonian (1) is modeled by the coupled two-HO model, and can be further rewritten in a time-independent form in the rotating framework as


with the detuning . In the derivation of the above Hamiltonian, we have used the rotating wave approximation (RWA) when (where ), which is always fulfilled for most realistic atoms.

Sideband cooling for atomic collective excitations.- Generally, the atomic collective-excitation modes have non-vanishing mean thermal populations due to their couplings to the bath at finite temperature. In experiments, the frequency of the higher-frequency atomic collective-excitation, i.e., mode , is of the order of Hz, which implies that its mean thermal excitation number can be considered as zero even at room temperature. Usually, the atomic ground state and meta-stable one are selected as the atomic two hyperfine levels with the frequency difference being the order of Hz. Although there is no optical dipole transition between and because of the electric dipole transition rule, the decay from to still exists due to the atomic collision or some other cases, with a very low decay rate. Such a very-low decay rate means that the lower-energy mode possesses a long coherence time, which is just a distinct advantage of using the atomic collective excitations as quantum memory units. However, in consideration of the high initial mean thermal population at room temperature K (with the Boltzmann constant), it is necessary to cool the atomic collective-excitation modes to their ground states before quantum information processing based on atomic collective excitations.

In the presence of noises, we may have the following Langevin equation from Hamiltonian (2)


where (), and . The noise operators are described by the correlations . Here, are the decay rates of collective-excitation modes and , respectively (for simplicity, we adopt the same symbols as those of the atomic levels and ), and are the corresponding initial thermal populations with the initial temperature of the thermal bath. Although the above quantum Langevin equation has vanishing steady state solutions , the corresponding quantum rate equations for the excitation numbers () read


where and . Here we have used the non-vanishing noise-based relations (22) .

The steady state solutions of the quantum rate equations give the variation of final mean population with

Then, from the Bose-Einstein distribution, the effective temperature of mode is expressed as


For a simple case of (namely, the driving light is exactly resonant to the atomic transition : ), the nice cooling reaches with


in the strong driving strength limit . For a realistic atomic system, one has and (). Especially, when is sufficiently small such that  (23), the final mean population reaches its limit: .

As mentioned above, the mean thermal population of mode is usually tiny, which means that the atomic collective-excitation mode can be cooled close to its ground state with the final thermal population .

A physical explanation of the above results can resort to the sideband-cooling-like mechanism (see Fig. 1(b)). The Jaynes-Cummings (JC) term () causes the anti-Stokes transition from to , which will decay fast to the state . Thus, such a process makes the lower-frequency oscillator to lose one quantum and then results in its cooling. When the anti-Stokes transition is resonantly coupled, namely, , or , the best cooling happens with the corresponding optimal final mean population () given by the initial population of higher-frequency mode . All in all, in order to reach the optimal cooling of lower-energy collective-excitation mode , the following conditions should be satisfied: (i) strong enough pumping light ; (ii) the resonantly driving condition: ; (iii) and (that is, ). It is notable that the above three conditions can be met for experimentally accessible parameters of realistic atomic systems (23).

It is seen clearly from the above analysis that the time-dependent coupling between two large-detuned HOs could cool down the lower-frequency one. This cooling model is different from the existing mechanical cooling scheme based on the optical radiation pressure (12); (13); (14); (15); (16), with an external laser-driving. Nevertheless, we will show below that these two cooling schemes may be generalized to a more universal model.

Generalized sideband cooling model of two coupled HOs.- A naive cooling process could be realized when a hotter object contacts directly with a cold one. If there exists no external driving for two objects at the same initial temperature, it is obviously impossible that the temperature of any one can change via their direct interaction. But the situation changes dramatically when we add an additional time-dependent driving or manipulate the coupling between them to be time-dependent in largely-detuned two coupled HOs. This kind of setup leads to a more general sideband cooling framework.

Figure 2: (Color online) Coupled two HOs ( and ) model. is the desired lower-frequency HO to be cooled. (a) The interaction between the HOs is time-dependent modulated (); (b) The coupling strength of the interaction between two HOs is time-independent but there is an external time-dependent driving () on the higher-frequency mode .

Let us first consider two coupled HOs with large-detuned frequencies () as seen in Fig. 2(a). The free Hamiltonian reads . A time-dependent coupling is generally expressed as , where () and () are the creation (annihilation) operators of the oscillators and with the coupling coefficient between them and the modulating frequency. Here, is a function of operators and . For simplicity, in what follows we consider only the simplest case of , though a more general function (i.e., with dimensionless coefficients) would lead to a similar result. In the time-varying frame reference defined by , the effective Hamiltonian of the coupled system reads


where the high-oscillating terms have been neglected and the detuning could be negative when .

Next we consider another type of two-HO system (see Fig. 2 (b)): a general time-independent interaction is with the coupling strength and being Hermitian, and a periodically driving field on the higher-frequency HO reads . In the time-varying frame reference defined by , the total Hamiltonian reads with after neglecting the high-oscillating terms, where keeps the time-independent terms in . Around some quasi-classical state such that and , the quantum dynamics is determined by an effective Hamiltonian with the displacement operators and for quantum fluctuations. Then, when the displacements and take the equilibrium values and , the effective Hamiltonian has the same form as that given in Eq. (8) with the parameters and . Therefore, these types of coupled two-HO model should have the same cooling mechanism to cool the lower-frequency HO mode.

We wish to point out that the optical radiation-pressure cooling of mechanical resonator (13); (14); (15); (16), is just a special case of the second type with . A similar linearization (13); (16) of the effective Hamiltonian as given in Eq. (8) was also mentioned in the optical radiation-pressure cooling of mechanical resonator. Here we present only the cooling limit (so-called sideband cooling limit) (24) of the general coupled two-HO model:


in the resolved sideband case when . Here the usual relation has been used.

Although the above Hamiltonian (8) describes only a simple coupled two-HO system, it can capture the essence of almost all sideband cooling schemes. We need to emphasize the necessarity of the time-dependence of modulating coupling or external driving. It lies in a fact that, when , there still exists the effective interaction for  (or ). It is the effective resonance that results in the sideband transitions to cool down (or heat up) the oscillator (see Fig. 1(b) and (c)): the JC term () (associated with the fast decay of mode ) denotes the cooling process of lower-frequency oscillator (); on the contrary, the anti-JC term (that is, the anti-rotating term) () denotes the heating process of mode (). When the cooling process dominates (e.g., when ), the cooling of mode happens with the optimal cooling subject to the usual sideband cooling limit ().

Comparing the cooling models described by the Hamiltonians (2) and (8), it is clear that the anti-JC terms () are absent in the former describing the atomic ensemble. Thus, due to absence of the heating process induced by the anti-JC term during the resolved sideband cooling, the optimal cooling of lower-frequency collective-excitation happens at the exact resonant () of (first) anti-Stokes transitions and the corresponding cooling limit () is certainly much less than that of the usual sideband cooling limit ().

Conclusion.- We have established a theory to cool atomic collective excitations in an optically-driven three-level atomic ensemble. Such a cooling protocol is quite useful and promising in quantum information processing based on atomic collective excitations, which breaks the usual sideband cooling limit. Moreover, motivated by the optical radiation-pressure cooling scheme of mechanical oscillator, we have also proposed two generalized cooling types of the coupled two-HO model: the first one possesses a time-dependent modulating coupling coefficient between the HOs without the external driving; while for the second one, an additional external time-dependent driving on the higher-frequency HO is involved, with the coupling coefficient between the HOs being time-independent. In fact, the second type is a generalized model of the optical radiation-pressure cooling of mechanical resonator. For both types, the lower-frequency HO can be cooled in the resolved sideband cooling case with the usual sideband cooling limit.

This work was supported by the RGC of Hong Kong under Grant No. HKU7051/06P, and partially supported by the NFRP of China under Grant Nos. 10874091 and 2006CB921205 and NSFC Grants through ITP, CAS.


  1. M. Fleischhauer and M. D. Lukin, Phys. Rev. Lett. 84, 5094 (2000); Phys. Rev. A 65, 022314 (2002).
  2. K.-J. Boller, A. Imamolu, and S. E. Harris, Phys. Rev. Lett. 66, 2593 (1991); S. E. Harris, Phys. Today 50, No. 7, 36 (1997); M. Xiao et al., Phys. Rev. Lett. 74, 666 (1995); H. Wu et al., Phys. Rev. Lett. 100, 173602 (2008).
  3. C. P. Sun, Y. Li, and X. F. Liu, Phys. Rev. Lett. 91, 147903 (2003); Y. Li and C. P. Sun, Phys. Rev. A 69, 051802(R) (2004).
  4. M. Fleischhauer, A. Imamoglu, and J. P. Marangos, Rev. Mod. Phys. 77, 633 (2005).
  5. L.-M. Duan, M. D. Lukin, J. I. Cirac, and P. Zoller, Nature 414, 413 (2001).
  6. A. Kuzmich et al., Nature 423, 731 (2003); C. W. Chou et al., Science 316, 1316 (2007).
  7. B. Julsgaard et al., Nature 432, 482 (2004); M. D. Eisaman et al., Nature 438, 837 (2005).
  8. C. Liu et al., Nature 409, 490 (2001).
  9. B. Zhao et al., Phys. Rev. Lett. 98, 240502 (2007).
  10. A. N. Clelandand and M. L. Roukes, Appl. Phys. Lett. 69, 2653 (1996); X. M. H. Huang et al., Nature 421, 496 (2003).
  11. I. Wilson-Rae et al., Phys. Rev. Lett. 92, 075507 (2004); P. Zhang et al., Phys. Rev. Lett. 95, 097204 (2005); A. Naik et al., Nature 443, 193 (2006).
  12. C. H. Metzger and K. Karrai, Nature (London) 432, 1002 (2004); S. Gigan, et al., Nature (London) 444, 67 (2006); O. Arcizet et al., Nature (London) 444, 71 (2006);
  13. I. Wilson-Rae et al., Phys. Rev. Lett. 99, 093901 (2007); T. J. Kippenberg and K. J. Vahala, Opt. Express 15, 17172 (2007).
  14. F. Marquardt et al., Phys. Rev. Lett. 99, 093902 (2007); F. Marquardt et al., J. Mod. Opt. 55, 3329 (2008).
  15. C. Genes et al., Phys. Rev. A 77, 033804 (2008); Y. Li et al., 78, 134301 (2008); M. Grajcar et al., Phys. Rev. B 78, 035406 (2008).
  16. P. Rabl, C. Genes, K. Hammerer, and M. Aspelmeyer, arXiv: 0903.1637; S. Gröblacher, K. Hammerer, M. R. Vanner, M. Aspelmeyer, arXiv: 0903.5293.
  17. M. D. LaHaye, O. Buu, B. Camarota, and K. C. Schwab, Science 304, 74 (2004).
  18. F. Diedrich et al., Phys. Rev. Lett. 62, 403 (1989); C. Monroe et al., Phys. Rev. Lett. 75, 4011 (1995).
  19. S. E. Hamann et al., Phys. Rev. Lett. 80, 4149 (1998).
  20. S. Chu, Science 253, 861 (1991); C. S. Wood et al., Science 275, 1759 (1997).
  21. G. R. Jin et al., Phys. Rev. B 68, 134301 (2003).
  22. M. O. Scully and M. S. Zubairy, Quantum Optics, Chap. 9 (Cambridge Univercity Press, New York, 1997).
  23. For typical alkali-(like)-metal -type atoms, Hz, Hz, Hz, Hz (See Refs. (2); (8); (25) and references therein). The condition may be fulfilled for Hz.
  24. For detailed calculations, one may refer to those in (13); (14); (15).
  25. A. Mosk et al., Appl. Phys. B 73, 791 (2001).
Comments 0
Request Comment
You are adding the first comment!
How to quickly get a good reply:
  • Give credit where it’s due by listing out the positive aspects of a paper before getting into which changes should be made.
  • Be specific in your critique, and provide supporting evidence with appropriate references to substantiate general statements.
  • Your comment should inspire ideas to flow and help the author improves the paper.

The better we are at sharing our knowledge with each other, the faster we move forward.
The feedback must be of minumum 40 characters
Add comment
Loading ...
This is a comment super asjknd jkasnjk adsnkj
The feedback must be of minumum 40 characters
The feedback must be of minumum 40 characters

You are asking your first question!
How to quickly get a good answer:
  • Keep your question short and to the point
  • Check for grammar or spelling errors.
  • Phrase it like a question
Test description