Tension mediated nonlinear coupling between orthogonal mechanical modes of nanowire resonators
We study the nonlinear coupling between orthogonal flexural modes of doubly clamped InAs nanowire resonators. The two orthogonal modes are formed by the symmetry breaking and lifting of degeneracy of the fundamental mode. The presence of a Duffing nonlinearity emerges when a mode is driven to large amplitudes. In this regime the modes are coupled due to the tension induced from the large amplitude of oscillations and is reflected in the hysteretic response of the mode that is not strongly driven. We study the driven-driven response of the mechanical modes to elucidate the role of nonlinear mode coupling in such mechanical resonators. The dynamics of the coupled modes studied here could prove useful in technological applications such as nanowire based vectorial force sensing.
Understanding the coupling between different modes of a complex system is of great interest as it can be used to improve functionality such as enhancing the sensitivity of the system. Optomechanics, for example, has harnessed the coupling between a mechanical oscillator and an optical cavity aspelmeyer_cavity_2014 () to explore the limits of precise position measurements. Similarly, the coupling between two vibrational modes of nanomechanical systems has also been explored in recent times.
Coupling between mechanical modes has been studied in nanofabricated doubly clamped beams mahboob_phonon-cavity_2012 (); okamoto_coherent_2013 (); faust_nonadiabatic_2012 (), nanofabricated cantilevers westra_interactions_2011 (); westra_nonlinear_2010 (), carbon nanotubes castellanos-gomez_strong_2012 (); eichler2012strong (), 2D materials alba_tunable_2016 (); mathew_dynamical_2016 (); liu_optical_2015 (), cantilevers of VLS (vapour liquid solid) grown nanowires cadeddu_time-resolved_2016 (); lepinay_universal_2016 (); foster_tuning_2016 (); rossi_vectorial_2016 () and doubly clamped VLS nanowires solanki_tuning_2010 (). The origin of nonlinear intermodal coupling can be complex and system specific lifshitz2008nonlinear (); khan_tension-induced_2013 (); eriksson_frequency_2013 (); efforts to understand the microscopic origin are ongoing across systems as tunability of this nonlinear coupling can provide additional functionality to devices.
VLS grown nanowires dasgupta_25th_2014 () offer advantage of engineering the properties with unprecedented control algra_twinning_2008 (); johansson_controlled_2009 (). Recently, orthogonal vibrational modes of the cantilevers, singly clamped nanowires, made using VLS grown nanowires have been used to vectorially map lepinay_universal_2016 (); rossi_vectorial_2016 () the forces on a surface to provide maps of electric fields. The two orthogonal vibrational modes arise due to an unintentional breaking of symmetry of the degenerate fundamental mode. This pair of modes can provide complementary information about the nano electromechanical system (NEMS) and are, hence, of interest. We show that the Duffing nonlinearity of a mode that is driven to large amplitudes imprints itself as a hysteretic increase in frequency of the second mode. In this paper, we study in detail the inter-modal nonlinear coupling and show that it can be large and tunable as a function of the tension in the nanowires. Tunability due to tension is absent in singly clamped beams where nonlinear coupling has been studied recently cadeddu_time-resolved_2016 (). We compare the strength of coupling across systems and find that the coupling in our system is large and comparable to the coupling observed in carbon nanotube resonators. In addition, the key role of tension mediated intermodal coupling is demonstrated by the fact that the strength of the coupling in our doubly clamped nanowire devices is significantly larger than cantilever devices made using nanowires. The microscopic model we develop explains the experimental observations accurately.
Ii Experimental methods
We start by briefly describing the nanofabrication of devices used in our experiments; details of fabrication are available in previous reports solanki_tuning_2010 (); abhilash2012 (). InAs nanowires of 10 m length and 100 nm diameter were grown using MOCVD techniques. Intrinsic silicon wafers with 100 nm of thermally grown nitride were used as the substrate for device fabrication. A thin layer of electron beam (e-beam) resist was spun on the substrate. The thickness of this resist layer decides the height above the substrate by which the nanowire is suspended. The nanowires were removed from the growth substrate and then drop cast above the e-beam resist coated substrate and then covered by additional layers of e-beam resists. After patterning source, drain, and gate electrodes using standard e-beam lithography, the substrate was loaded in to a sputtering system with an in-situ plasma etcher for conformal deposition of metal. Prior to metal deposition the sample was exposed to an argon plasma to remove the residual oxide on the nanowires. This allows the formation of Ohmic contact to the nanowire. Gold was sputtered on the substrate preceded by a thin layer of chromium for adhesion. The sputtered metal forms both the electrical contacts as well as mechanical anchors for suspending the device. Lift-off followed by drying the substrate completes the device fabrication process.
Figure 1 shows a false colored scanning electron microscope (SEM) image of a device along with the schematic of the circuit used in our experiments. The insulating nature of the intrinsic silicon substrates at low temperatures negates the effects of parasitic capacitances and allows us to carry out direct readout of the electrical signal at radio frequencies (rf)abhilash2012 (); xu2010radio (). DC and rf signals were combined using a bias tee and applied to the gate electrode to actuate the mechanical oscillations in the resonator. The change in rf current through the device due to mechanical oscillations were then measured by a vector network analyzer (VNA). The signal from the VNA was used to drive and probe one mechanical mode in the linear regime, while another signal combined from a function generator (FG) was used to drive and pump the second mode to large amplitude oscillations. This allows us to investigate the driven response of one mechanical mode to large amplitude oscillations of the second mode. All experiments were performed with sample temperature at 5 K.
Figure 2(a) shows the response of the nanowire resonator measured using the network analyzer with the pump signals turned off for an applied DC gate voltage of -20 V. The lower frequency mode at 59.5 MHz is seen to have a large signal compared to the higher mode at 60.9 MHz with quality factor of 2800 for both modes. Here, the amplitude of mode 1 at resonance is estimated to be 0.8 nm (see supplementary material) for a drive power of -30 dBm. For the remainder of the article we shall refer to the lower/higher frequency mode as mode 1/mode 2. The small frequency difference (1.4 MHz) between the two modes implies that they are not harmonics of the vibration, rather they correspond to the non-degenerate, orthogonal flexural modes of the resonator. These orthogonal modes are shown in the inset of Figure 2(a). The degeneracy of the orthogonal components of the fundamental mode can be broken by any asymmetry in the nanowire. Figure 2(b) shows the dispersion of the resonant modes with applied DC gate voltage. Mode 1 is seen to disperse negatively with increasing absolute value of the gate voltage. This is indicative of the capacitive softening kozinsky_tuning_2006 (); solanki_tuning_2010 () effect of mode 1. Mode 2, however, is seen to have negligible dispersion with the gate voltage. The observed dispersion of the two modes to an applied DC gate voltage is indicative of their plane of oscillations. We deduce that mode 1 oscillates mainly in the plane of the substrate as the capacitive softening effect occurs in nanoelectromechanical systems (NEMS) when the oscillations are in the plane of the gate electrode. Mode 2, therefore, oscillates in a nearly vertical plane perpendicular to the substrate. Here we note that the good visibility of the modes for negative gate voltages in Figure 2(b) arises due to the non-zero transconductance of the semiconductor nanowire. The n-type semiconducting character of the as grown nanowires is reflected in the visibility of the dispersion diagram (see supplementary material for gating response of the nanowires). In the following discussions we fix the gate voltage to -20 V and study the mechanical response of mode 1 to large amplitude oscillations of mode 2.
Iii Results and discussion
Figure 3 shows the effect of a large driving force on mode 2 on the frequency response of mode 1. Here the linear response of mode 1 is probed with a weak signal from the VNA with -30 dBm power whereas the pump frequency, around mode 2, is a strong signal from the FG such that mode 2 is driven in the nonlinear Duffing regime. Both the frequencies are swept in the increasing direction. For lower pump powers (0 dBm, left panel in Figure 3) where the resonant amplitude of mode 2 is estimated to be 23 nm (see supplementary material for detailed calculations), mode 1 frequency is seen to increase slightly when the pump frequency is in the vicinity of mode 2. As the pump power is increased to 10 dBm (right panel in Figure 3) mode 1 frequency is seen to be affected over larger range of the pump frequencies. As the pump frequency is increased mode 1 frequency is seen to gradually increase and abruptly decrease to its original value beyond a certain pump frequency. The observed response indicates that these orthogonal modes are nonlinearly coupled. We now explore the form of this nonlinear coupling further.
The leaning of the resonant frequency and subsequent, abrupt jump in the response is characteristic of the Duffing nonlinearity in these devices. The Duffing nonlinearity is characterized by presence of terms of the form in the equation of motion that gives rise to bistability in the responselifshitz2008nonlinear (). As the pump frequency matches mode 2, it drives mode 2 to large amplitudes until the point of bistability.
The response of mode 1, therefore, follows the Duffing response shape of mode 2. The frequency leaning of mode 1 arises from the deformation induced tension that accumulates on the nanowire as mode 2 oscillates with a large amplitude. The deformation induced tension is significant when the amplitude of oscillations becomes large. This tension can be written as
where is the Young’s modulus, and are the cross sectional area and length of the beam respectively, and is the mode shape as a function of the distance along the length of the nanowire. The mode shape can be written in terms of the in-plane, , and out-of-plane, , components for mode 1 and mode 2 respectively. Then the governing partial differential equations of motion for each mode will include a term of the formnayfeh2008nonlinear () (see supplementary material for full Euler-Bernoulli equations)
where is either or .
Along with the frequency leaning that accompanies the Duffing response, the bistable nature also gives rise to hysteresis in the response of a single mode with the direction of frequency sweeps. As the modes are coupled, we expect the hysteretic Duffing response of the pumped mode to reflect in the response of the probed mode as well. Figure 4 shows the effect of pump sweep direction on the response of mode 1. The coupled response of mode 1 faithfully mimics the Duffing response of mode 2.
To arrive at equation 3 we have used a reduced order technique to solve the coupled partial differential equations (as described by Euler-Bernoulli theory) that govern the dynamics of our system. The factors where is the non-dimensional coefficient of nonlinear modal interaction governed by the geometry of the device (see supplementary material for details). The above equations of motion capture all the physics of our system. We solve these equations numerically to compare with the experimentally observed results. The bottom panels in Figures 3-4 show the simulated response of the nanowire resonator for corresponding experimental data in the top panels. The calculated response is seen to match well with the experimentally observed frequency shifts, bistability, and hysteresis.
In order to understand and compare our experiments with similar systems studied earlier we compare the key parameters in Table 1. denotes the frequency of the lower of the two coupled modes, is difference in the frequency of the modes and is the rate of change of frequency of the un-pumped mode as a function of the pumped mode. Larger the nonlinear coupling larger is and to first order the slope of the nonlinear coupling induced response is linear; this is seen in Figure 3(b) and Figure 4(a). We find that the extent of nonlinear coupling is much larger in doubly clamped nanomechanical devices and this attests to the key role of tension in mediating the nonlinear coupling. Naturally, such a strong nonlinear coupling is not present in cantilevers made using nanowires cadeddu_time-resolved_2016 (). We also find, from our calculations, that the coupling is the strongest between the two orthogonal modes of the fundamental (details provided in the supplementary material). It would be interesting to explore parametric degenerate and nondegenerate amplification using such coupled modes mathew_dynamical_2016 (). Especially since nanowire based vectorial AFM lepinay_universal_2016 (); rossi_vectorial_2016 () has been demonstrated using parametric schemes for these coupled modes could help push sensitivity to new limits in vectorial scanning.
|Carbon nanotubescastellanos-gomez_strong_2012 () (Castellanos-Gomez et al.)||180 MHz||730 MHz||1|
|Nanofabricated doubly clamped beams westra_nonlinear_2010 () (Westra et al.)||275 kHz||200 kHz||1|
|VLS grown nanowires cantilevers cadeddu_time-resolved_2016 () (Cadeddu et al.)||1 MHz||6 kHz||0.1|
|VLS grown doubly clamped nanowires (present work)||50 MHz||1.6 MHz||0.8|
In summary, we have studied the tension mediated nonlinear coupling between the orthogonal modes of an InAs nanowire resonator. Our experiments show that the Duffing nonlinearity of one mode affects the linear response of the second mode as observed from the abrupt and hysteretic frequency shifts. Our calculations deduce the role of large-oscillation induced tension on the observed dynamics of the system. Such coupled dynamics could be exploited to improve the performance and bandwidth of NEMS based sensors.
We acknowledge the contribution of Mr. Mahesh Gokhale and Professor Arnab Bhattacharya, TIFR, for growth of the nanowires. We acknowledge funding from the Swarnajayanti Fellowship of DST (for MMD), Department of Atomic Energy, and Department of Science and Technology of the Government of India through the Nanomission. A.B. acknowledges the Science and Engineering Research Board, Government of India for funding.
- (1) M. Aspelmeyer, T. J. Kippenberg, F. Marquardt, Cavity optomechanics, Reviews of Modern Physics 86 (4) (2014) 1391–1452.
- (2) I. Mahboob, K. Nishiguchi, H. Okamoto, H. Yamaguchi, Phonon-cavity electromechanics, Nature Physics 8 (5) (2012) 387–392.
- (3) H. Okamoto, A. Gourgout, C.-Y. Chang, K. Onomitsu, I. Mahboob, E. Y. Chang, H. Yamaguchi, Coherent phonon manipulation in coupled mechanical resonators, Nature Physics 9 (8) (2013) 480–484.
- (4) T. Faust, J. Rieger, M. J. Seitner, P. Krenn, J. P. Kotthaus, E. M. Weig, Nonadiabatic Dynamics of Two Strongly Coupled Nanomechanical Resonator Modes, Physical Review Letters 109 (3) (2012) 037205.
- (5) H. J. R. Westra, D. M. Karabacak, S. H. Brongersma, M. Crego-Calama, H. S. J. van der Zant, W. J. Venstra, Interactions between directly- and parametrically-driven vibration modes in a micromechanical resonator, Physical Review B 84 (13) (2011) 134305.
- (6) H. J. R. Westra, M. Poot, H. S. J. van der Zant, W. J. Venstra, Nonlinear Modal Interactions in Clamped-Clamped Mechanical Resonators, Physical Review Letters 105 (11) (2010) 117205.
- (7) A. Castellanos-Gomez, H. B. Meerwaldt, W. J. Venstra, H. S. J. van der Zant, G. A. Steele, Strong and tunable mode coupling in carbon nanotube resonators, Physical Review B 86 (4) (2012) 041402.
- (8) A. Eichler, M. del Álamo Ruiz, J. Plaza, A. Bachtold, Strong coupling between mechanical modes in a nanotube resonator, Physical Review Letters 109 (2) (2012) 025503.
- (9) R. D. Alba, F. Massel, I. R. Storch, T. S. Abhilash, A. Hui, P. L. McEuen, H. G. Craighead, J. M. Parpia, Tunable phonon-cavity coupling in graphene membranes, Nature Nanotechnology 11 (9) (2016) 741–746.
- (10) J. P. Mathew, R. N. Patel, A. Borah, R. Vijay, M. M. Deshmukh, Dynamical strong coupling and parametric amplification of mechanical modes of graphene drums, Nature Nanotechnology 11 (9) (2016) 747–751.
- (11) C.-H. Liu, I. S. Kim, L. J. Lauhon, Optical Control of Mechanical Mode-Coupling within a MoS Resonator in the Strong-Coupling Regime, Nano Letters 15 (10) (2015) 6727–6731.
- (12) D. Cadeddu, F. R. Braakman, G. Tütüncüoglu, F. Matteini, D. Rüffer, A. Fontcuberta i Morral, M. Poggio, Time-Resolved Nonlinear Coupling between Orthogonal Flexural Modes of a Pristine GaAs Nanowire, Nano Letters 16 (2) (2016) 926–931.
- (13) L. M. d. Léffpinay, B. Pigeau, B. Besga, P. Vincent, P. Poncharal, O. Arcizet, A universal and ultrasensitive vectorial nanomechanical sensor for imaging 2d force fields, Nature Nanotechnology 12 (2) (2016) 156–162.
- (14) A. P. Foster, J. K. Maguire, J. P. Bradley, T. P. Lyons, A. B. Krysa, A. M. Fox, M. S. Skolnick, L. R. Wilson, Tuning Nonlinear Mechanical Mode Coupling in GaAs Nanowires Using Cross-Section Morphology Control, Nano Letters 16 (12) (2016) 7414–7420.
- (15) N. Rossi, F. R. Braakman, D. Cadeddu, D. Vasyukov, G. Tütüncüoglu, A. F. i. Morral, M. Poggio, Vectorial scanning force microscopy using a nanowire sensor, Nature Nanotechnology 12 (2) (2016) 150–155.
- (16) H. S. Solanki, S. Sengupta, S. Dhara, V. Singh, S. Patil, R. Dhall, J. Parpia, A. Bhattacharya, M. M. Deshmukh, Tuning mechanical modes and influence of charge screening in nanowire resonators, Physical Review B 81 (11) (2010) 115459.
- (17) R. Lifshitz, M. Cross, Nonlinear dynamics of nanomechanical and micromechanical resonators, Review of nonlinear dynamics and complexity 1 (2008) 1–52.
- (18) R. Khan, F. Massel, T. T. Heikkilä, Tension-induced nonlinearities of flexural modes in nanomechanical resonators, Physical Review B 87 (23) (2013) 235406.
- (19) A. M. Eriksson, D. Midtvedt, A. Croy, A. Isacsson, Frequency tuning, nonlinearities and mode coupling in circular mechanical graphene resonators, Nanotechnology 24 (39) (2013) 395702.
- (20) N. P. Dasgupta, J. Sun, C. Liu, S. Brittman, S. C. Andrews, J. Lim, H. Gao, R. Yan, P. Yang, 25th Anniversary Article: Semiconductor Nanowires - Synthesis, Characterization, and Applications, Advanced Materials 26 (14) (2014) 2137–2184.
- (21) R. E. Algra, M. A. Verheijen, M. T. Borgström, L.-F. Feiner, G. Immink, W. J. P. van Enckevort, E. Vlieg, E. P. A. M. Bakkers, Twinning superlattices in indium phosphide nanowires, Nature 456 (2008) 369.
- (22) P. Caroff, K. A. Dick, J. Johansson, M. E. Messing, K. Deppert, L. Samuelson, Controlled polytypic and twin-plane superlattices in iii–v nanowires, Nature Nanotechnology 4 (1) (2009) 50–55.
- (23) T. Abhilash, J. P. Mathew, S. Sengupta, M. R. Gokhale, A. Bhattacharya, M. M. Deshmukh, Wide bandwidth nanowire electromechanics on insulating substrates at room temperature, Nano Letters 12 (12) (2012) 6432–6435.
- (24) Y. Xu, C. Chen, V. V. Deshpande, F. A. DiRenno, A. Gondarenko, D. B. Heinz, S. Liu, P. Kim, J. Hone, Radio frequency electrical transduction of graphene mechanical resonators, Applied Physics Letters 97 (24) (2010) 243111.
- (25) I. Kozinsky, H. W. C. Postma, I. Bargatin, M. L. Roukes, Tuning nonlinearity, dynamic range, and frequency of nanomechanical resonators, Applied Physics Letters 88 (25) (2006) 253101.
- (26) A. H. Nayfeh, D. T. Mook, Nonlinear oscillations, John Wiley & Sons, 2008.
Supplementary material: Tension mediated nonlinear coupling between orthogonal mechanical modes of nanowire resonators
Appendix S1 Mathematical modelling
We have performed numerical simulations to understand the mode coupling behaviour of InAs nanowire resonators. A nanowire can be modeled as cylindrical vibrating beam having same frequency in all direction of the planes of flexural vibration. But, in presence of small imperfection in cross-section, a single resonant frequency of the nanowire splits into two nearby frequencies in orthogonal principal planes santos2010 (). we have observed similar two nearby resonant frequencies in the experiments of the InAs nanowire. So, the InAs nanowire has been modelled as a wire of elliptical cross-section as shown in Figure S1. For electrostatic actuation, it is placed distance apart from a gate electrode. The nanowire has mass density , length , semi-major axis , and semi-minor axis ; further, the cross-section area is denoted as and principal flexural stiffnesses as and .
The flexural dynamics of the nanowire is described in terms of its displacements and along principal orthogonal directions (X-axis and Y-axis). Here, the variables and are distance coordinate along axis of the nanowire and time coordinate respectively. The purpose of using on variables name is to distinguish their dimensional form from their non-dimensional form which are introduced in this section later. Using Euler-Bernoulli beam theory, the flexural dynamics of the electrostatically actuated InAs nanowire is governed by following coupled partial differential equations conley2008 (); chen2010 (); bhushan ()
In Eq. (S1), the variable is introduced to account for viscous damping, whereas the purpose of the end force is to account for the presence of residual stress due to doubly-clamped or fixed boundaries. The nanowire is actuated by unit length forces and along x-direction and y-direction respectively. These forces build-up when we actuate the nanowire by providing DC and AC voltages between nanowire and the gate electrode. For simulations, we have assumed unit length force of an electrostatically actuated circular cross-section nanowire having radius as actuation force of the InAs nanowire. In case of a cylindrical nanowire, which has circular cross-section, the electrostatic actuation force is developed in the direction of gate electrode bhushan2014 ()
here is the displacement of the nanowire in direction of the gate electrode. The variable is the applied voltage between the nanowire and gate electrode and is vacuum permittivity. In view of experiments, we have two AC voltage excitations corresponding to probe frequency and pump frequency along with the DC voltage, . During simulation, we have approximated to compute unit length forces along x-direction and along y-direction. We have assumed the major and minor axes of the elliptical cross-section of nanowire are inclined with respect to direction of the gate electrode (refer Fig. S1). The forces and are components of actuation force of a cylindrical nanowire, where and are constants.
For simplicity, we have transformed Eq. (S1) in non-dimensional form by introducing following non-dimensional variables defined as , , , and ( is a time constant). The non-dimensional form of Eq. S1 is
In Eq. (S3), the notations and denote partial derivative with respect to and respectively. In Eq. (S3), is the non-dimensional form of the end force and the variable is the ratio of principal flexural stiffnesses. The non-dimensional coefficient quantifies nonlinear modal interaction behaviour in the nanowire flexural dynamics. The parameter is the non-dimensional damping coefficient. We have used the value of corresponding to experimental quality factor in numerical calculations. The non-dimensional unit length forces are denoted by and .
We have solved Eq. (S3) using Galerkin based reduced order model technique bhushan2014 (); bhushan (). The solution of Eq. (S3) has been assumed in form of
Here, and are mode shapes along principal directions corresponding to fundamental nearby natural frequencies, whereas and are modal coordinate displacements. The modeshape (along x-direction) has been calculated by solving characteristic equation and modeshape (along y-direction) has been calculated by solving . Here, and are the two nearby fundamental natural frequencies. The assumed solution (S4) has been substituted in Eq. (S3), multiplied the equations with modeshapes, and integrated the equations from 0 to 1; we get
Various coefficients of the nonlinear terms of Eq. (S5) are
In Eq. (S5), the values of electrostatic actuation forces are and . By Taylor series expansion of the function (S2) of electrostatic forcing, one can deduce that electrostatic forcing functions and have first harmonic excitation terms, second harmonic excitation terms, and parametric excitation terms. It is because Eq. (S5) is a function of displacement coordinates and due to presence of square of voltage , where has both DC and AC voltage components. But, when investigation is near fundamental natural frequency and the gap distance between the nanowire and gate electrode is relatively larger bhushan2014 (); bhushan (); conley2008 (), first harmonic excitation term has dominant effect. So, we retain only first harmonic excitation term in electrostatic actuation force as
As the driving force increases, the amplitude of the modes increase giving rise to mode coupling. The amplitude of motion of the modes can be estimated by using the expression for the electrostatic driving force given in Eq. S2. By approximating the displacement of the nanowire to be small compared to the gate electrode separation, the total amplitude of the driving force acting along the length of the nanowire can be written as
For a linear response, the amplitude of motion on resonance is then given by , where is the mass of the nanowire and is the frequency of the mode. Using the dimensions of suspended length m, semi-minor axis nm, semi-major axis nm, initial gap nm, and quality factor , the amplitude can be estimated to be 0.8 nm for mode 1 for a drive power of -30 dBm, and 23 nm for mode 2 for a drive power of 0 dBm and DC gate voltage of 20 V.
Appendix S2 Numerical simulation
We have solved Eq. (S5) to understand mode coupling behaviour of the InAs nanowire resonator. The nanowire resonator was simulated using the dimenions given above and an end force as built-in tension of magnitude 1.47 times first Euler-buckling load. We have chosen the values of and near experimentally measured radius of the nanowire, along with , such that the nanowire has nearly same experimentally measured split resonant frequencies. In simulations, we actuate the nanowire with DC voltage = 20 V and vary magnitude of AC voltages and to investigate resonance behaviour. Figures S2(a) and S2(b) show the resonance behaviour around split resonant frequencies; here the lower and higher frequency modes are referred as mode 1 and mode 2 respectively. To obtain resonance in mode 1 oscillation, as shown in Fig. S2(a), we provide small magnitude of first AC voltage V in absence of second AC voltage V. Similarly, for resonance in mode 2 oscillation, as shown in Fig. S2(b), we provide second AC voltage V in absence of first AC voltage V. The line shape of these resonance curves demonstrate that they are linear in nature, and it is due to small magnitude of harmonic excitation. However, the nanowire resonator is inherently nonlinear in nature due to doubly-clamped boundary conditions, and nonlinearity is accounted in the equation of motion (S5) with Duffing nonlinearity terms. The nonlinearity effects become dominant in resonance behaviour at higher amplitude of harmonic AC voltage excitation. Figures S3(a) and S3(b) depict nonlinear resonance curves of mode 2 oscillation of the nanowire. Here, we actuate the nanowire with higher magnitude of second AC voltage V in absence of first AC voltage V.
The amplitude of AC voltage excitation is same for both Figs. S3(a) and S3(b), but direction of frequency sweep of AC voltage is different. In Fig. S3(a), the frequency sweep is in forward direction, whereas it is in reverse direction for Fig. S3(b). The resonance curves show hysteresis behaviour with change in direction of frequency sweep and it reflects the presence of nonlinearity.
Till now, we have discussed resonance in mode 1 and mode 2 oscillations separately by providing single input AC voltage corresponding to either mode 1 frequency or mode 2 frequency in absence of other. Now, we discuss the mode coupling behaviour in the InAs nanowire by simultaneously actuating both mode 1 and mode 2 by providing both first and second AC voltages. Figures S4(a) and S4(b) show mode 1 resonance behaviour of the nanowire when we actuate both first and second AC voltages. Here mode 1 is probed with a small magnitude of first AC voltage V, and second AC voltage actuation is a pump signal. Figure S4(a) shows mode 1 resonance for small magnitude of pump signal V. We can observe that there is shift in mode 1 resonant frequency with increase in magnitude of pump signal to V, as shown in Fig. S4(b). In both figures, excitation frequency of pump signal is 61 MHz. We explain the frequency shift in a simplified manner in the following way. When a nanowire is placed in an undeflected position, the axial force present in the nanowire is only due to the residual stress. During oscillation, additional axial force is developed in the nanowire due to deflection under restrained boundaries, and it is measured by following nonlinear coupling factor in Eq. (S3)
The motion of the nanowire along one mode influences the motion along other mode due to this nonlinear coupling factor. In Eq. (S3), first equation mainly governs mode 1 oscillation, whereas second equation governs mode 2 oscillation. When we pump mode 2 with high magnitude of AC voltage (refer second equation of Eq. (S3)), oscillatory motion in mode 2 vibration is set-up. The modal displacement of mode 2, , has harmonic response at the pump frequency as , where is amplitude of oscillation. Due to mode 2 oscillation, the additional axial force developed in the nanowire is proportional to square of or or . The additional axial force affects the mode 1 resonance due to presence of the nonlinear coupling factor (S6). Hence, the constant component of additional axial force, proportional to , adds up with the residual axial load and eventually shifts the resonant frequency of mode 1 vibration (refer first equation of Eq. (S5)).
Appendix S3 Analytical solution
We provide analytical expressions for computing the resonant frequency shift in probe mode oscillation. The magnitude of this resonant frequency shift can be computed by expression
Further, the amplitude of mode 2 oscillation can be obtained analytically by solving equation of motion using perturbation method under following approximations. In the present investigation, mode 1 is excited with a low magnitude AC voltage in comparison to mode 2 excitation. So, when we solve Eq. (S5), the effect of mode 1 vibration is negligible in computation of amplitude of mode 2, . We have solved the second equation of Eq. (S5), after ignoring coupling terms , using the perturbation technique, method of multiple scales nayfeh2008nonlinear (). The perturbation solution can be presented as a frequency response equation to compute the amplitude as a function of frequency difference in pump signal , and it is given by
Hence, by solving Eqs. (S7) and (S8), we can obtain probe signal frequency shift as a function of pump signal frequency difference .
We present the effectiveness of Eqs. (S7) and (S8) in computation of frequency shift using Figs. S5(a) and (b). Here, Fig. S5(a) shows nonlinear resonance behaviour of mode 2 oscillation when magnitude of pump signal or second AC voltage V; it is obtained by solving Eq. (S8). By comparing Fig. S5(a) with Figs. S3(a) and (b), we can say that perturbation solution (S8) is in good agreement with numerical solution of Eq. (S5). We have further computed frequency shift using solution of Eq. (S8) and Eq. (S7), and the solution is presented here in Fig. S5(b) by showing relationship between and . In this figure, we have also compared the analytical solution of Eq. (S7) with the numerical solution of Eq. (S5). There is good agreement between both solutions, and it demonstrates that the analytical expressions can serve as useful tool for computing frequency shift .
In this work, modal interaction between first planar and first nonplanar modes of vibration has been investigated. However, researchers have earlier investigated similar modal interaction between first planar and higher planar modes westra2010 (); gomez2012 (); westra2011 (). The derived expressions Eqs. (S7) and (S8) are also useful for obtaining the relationship between probe mode frequency shift (first planar mode) and pump mode frequency difference (higher planar mode). The motion of such a system is only governed by the first equation of Eq. (S3) because modal interaction between only planar modes are under consideration. From Eq. (S3), we get a system of two second order ordinary differential equations like Eq. (S5) by following Galerkin procedure as applied for derivation of Eq. (S5). Further, Eqs. (S7) and (S8) are applicable to obtain relationship between and .
To compare the modal interaction between different modes using Eqs. (S7) and (S8) we define a tuning constant which approximately quantifies relative coupling strength in modal interaction. The motivation in defining this constant is as follow. We can expand expression Eq. (S7) using Taylor series expansion and retain only linear term, and get that is directly proportional to and . In linear resonance case, the amplitude at resonance is directly proportional to and inversely proportional to and . Next, we have computed tuning constant for different cases of modal interaction in Table 1. Here, we consider three cases of modal interaction for first planar mode with first nonplanar mode (Type 1), first planar mode with second planar mode (Type 2), and first planar mode with third planar mode (Type 3). It is interesting that tuning constant is highest for the case of Type 1 modal interaction. The tuning constant for Type 2 modal interaction is zero due to antisymmetric nature of second mode which makes . We can also deduce from Table 1 that tuning constant for Type 1 modal interaction is about 2.65 times greater than Type 3 modal interaction.
|First planar and||First planar and||First planar and|
|first nonplanar||second planar||third planar|
|(Type 1)||(Type 2)||(Type 3)|
Relationship between and for case of Type 1 modal interaction is already shown in Fig. S5(b). We have further solved Eqs.(S7) and (S8) for investigating interaction of Type 3 modal interaction. We present the solution here in Figs. S6(a) and (b). Here, Fig. S6(a) shows nonlinear resonance behaviour of third planar mode oscillation when magnitude of pump signal or second AC voltage V as in case for Fig. S5(a). Further, the relationship between and for Type 3 modal interaction is shown in Fig. S6(b). Under similar loading condition, we can compare coupling strength of Type 1 and Type 3 modal interaction by observing Figs. S5(b) and S6(b). From these figures, we can deduce that tuning capacity (maximum value of ) in Type 1 modal interaction is about 2.65 times than Type 3 modal interaction. It is consistent with comparison of tuning constant of Type 1 and Type 3 modal interactions.
We can ascertain more information on Type 1 modal interaction by analyzing the expression for the tuning constant, . It provides insight on the frequency shift behaviour of the probe mode for varying magnitude of AC voltage of the pump mode . The maximum value of frequency shift is approximately proportional to the square of the magnitude of . This is because is proportional to the square of , and is proportional to . Figure S7 shows the calculated dependence of maximum frequency shift of probe mode on the magnitude of AC voltage of the pump mode.
Appendix S4 Gating response
The semiconducting nanowires used in this work are n-type in nature. As the conductance of the device depends on the carrier density in the nanowire the gate voltage can deplete or saturate the conductance (see Figure S8(a)). Therefore, as the nanowire undergoes mechanical oscillations the conductance of the device itself is modified due to the modulated gate capacitance. The conductance modulation due to oscillations is large when the transconductance of the device is large. Therefore, the strength of measured resonance signal depends on the transconductance.
Figure S8 shows the resonant response of mode 2 of the nanowire resonator at 20 V gate voltage showing the effect of a non-zero transconductance. As the magnitude of the gate voltage is same, the force acting on the resonator in both cases are equal. However, in regions (blue circle) where the transconductance of the device is high our measurement scheme is more effective in detecting the mechanical motion. Typical resonant response measured in experiments is seen in Figure S8(b) as a dip.
- (27) E. Gil-santos, D. Ramos, J. Martinez, M. Fernandez-Regulez, R. Garcia, A. S. Paulo, M. Calleja, J. Tamayo, Nanomechanical mass sensing and stiffness spectrometry based on two-dimensional vibrations of resonant nanowires, Nature Nanotechnology 5 (2010) 641–645.
- (28) W. G. Conley, A. Raman, C. M. Krousgrill, S. Mohammadi, Nonlinear and nonplanar dynamics of suspended nanotube and nanowire resonators, Nano Letters 8 (2008) 1590–1595.
- (29) Q. Chen, L. Huang, Y. Lai, C. Grebogi, D. Dietz, Extensively chaotic motion in electrostatically driven nanowires and applications, Nano Letters 10 (2010) 406–413.
- (30) A. Bhushan, M. M. Inamdar, D. N. Pawaskar, Effects of DC voltage on initiation of whirling motion of an electrostatically actuated nanowire oscillator, arXiv:1307.2359 [cond-mat.mes-hall].
- (31) A. Bhushan, M. M. Inamdar, D. N. Pawaskar, Simultaneous planar free and forced vibrations analysis of an electrostatically actuated beam oscillator, International Journal of Mechanical Sciences 82 (2014) 90–99.
- (32) A. H. Nayfeh, D. T. Mook, Nonlinear oscillations, John Wiley & Sons, 2008.
- (33) H. J. R. Westra, M. Poot, H. S. J. van der Zant, W. J. Venstra, Nonlinear modal interactions in clamped-clamped mechanical resonators, Physical Review Letters 105 (2010) 117205.
- (34) A. Castellanos-Gomez, H. B. Meerwaldt, W. J. Venstra, H. S. J. van der Zant, G. A. Steele, Strong and tunable mode coupling in carbon nanotube resonators, Physical Review B 86 (2012) 041402.
- (35) H. J. R. Westra, D. M. Karabacak, S. H. Brongersma, M. Crego-Calama, H. S. J. van der Zant, W. J. Venstra, Interactions between directly- and parametrically-driven vibration modes in a micromechanical resonator, Physical Review B 84 (2011) 134305.