One qubit and one photon – the simplest polaritonic heat engine

One qubit and one photon – the simplest polaritonic heat engine

Qiao Song Quantum Institute for Light and Atoms, School of Physics and Material Science, East China Normal University, Shanghai 200241, P.R. China    Swati Singh Department of Physics and College of Optical Sciences, University of Arizona, Tucson, Arizona 85721, USA Department of Physics, Williams College, Williamstown, MA 01267, USA    Keye Zhang kyzhang@phy.ecnu.edu.cn Quantum Institute for Light and Atoms, School of Physics and Material Science, East China Normal University, Shanghai 200241, P.R. China    Weiping Zhang Department of Physics and Astronomy, Shanghai Jiao Tong University, Shanghai, P.R. China Collaborative Innovation Center of Extreme Optics, Shanxi University, Taiyuan, Shanxi 030006, P. R. China    Pierre Meystre Department of Physics and College of Optical Sciences, University of Arizona, Tucson, Arizona 85721, USA American Physical Society, 1 Research Road, Ridge, NY 11961, USA
Abstract

Hybrid quantum systems can often be described in terms of polaritons. These are quasiparticles formed of superpositions of their constituents, with relative weights depending on some control parameter in their interaction. In many cases, these constituents are coupled to reservoirs at different temperatures. This suggests a general approach to the realization of polaritonic heat engines where a thermodynamic cycle is realized by tuning this control parameter. Here we discuss what is arguably the simplest such engine, a single qubit coupled to a single photon. We show that this system can extract work from feeble thermal microwave fields. We also propose a quantum measurement scheme of the work and evaluate its back-action on the operation of the engine.

pacs:
05.70.-a, 07.20.Pe, 42.50.Pq, 42.50.Dv

I Introduction

Experimental advances in single atom and ion manipulation and in nanofabrication have led to an increased interest in quantum thermodynamics, and more specifically in quantum heat engines (QHE) Uzdin2015 (). Abah and coworkers proposed Abah2012 (); Ronagel2014 () and demonstrated Rossnagel2016 () a scheme to realize a nanoscale QHE with a single ion. A trapped-ion system was also recently used An2014 () to carry out an experimental test of the quantum Jarzynski equality Jarzynski1997 (); Mukamel2003 (). Other approaches and related fundamental questions in quantum thermodynamics have been considered in systems ranging from quantum degenerate bosonic atoms Fialko2012 () to superconducting quantum circuits Quan2006 () and from macroscopically separated quantum-dot conductors coupled to a microwave cavity Bergenfeldt2014 () to atomic Scully2003 (); Scully2011 () or photon gases Hardal2015 () in optical resonators.

Many hybrid quantum systems can be conveniently described in terms of polaritons. These quasiparticles are quantum superpositions of the system constituents with relative weights that depend on some coupling parameter. The fact that these constituents are typically coupled to reservoirs at different temperatures suggests a general approach to the realization of quantum heat engines where a thermodynamic cycle is realized by periodically varying the control parameter. To an excellent approximation the nature of the quasiparticles is then changed from one to the other of their constituents, so that they are alternatively coupled to one or the other reservoir.

In previous work Zhang2014a (); Zhang2014b () we exploited this feature in a phonon polariton based optomechanical QHE Tercas2016 (). Here we expand the same idea to what is arguably the simplest such engine, a single two-state atom or artificial atom (e.g. a superconducting qubit) coupled to a single photon. In this case the polariton modes are the familiar dressed states of quantum optics Meystre2007 (). This system could be demonstrated experimentally in a circuit QED environment  Walraff2004 (); Blais2004 ().

The paper is organized as follows. Section II establishes our notation and outlines the quantum model of coupled qubit-photon system, including dissipation due to the the coupling of the qubit and the photon to a ‘cold’ and a ‘warm’ reservoir, respectively. Section III describes a quantum Otto cycle based on that qubit-photon system first for the simplest single-photon case, and then the multi-photon and the two-qubit cases. It also derives expressions for the work of the heat engine. Section IV discusses the parameters requirements of the engine working and designs a specific experimental realization based on the circuit QED system. Section V turns to measurement protocols of the work output. It compares explicitly the quantum backaction of dispersive and absorptive measurements on the statistics of the measured results. Finally, Section VI is a summary and outlook.

Figure 1: Solid lines: dressed qubit energy levels as a function of the qubit-field detuning with the qubit transition frequency and the cavity field frequency for . Dashed lines: corresponding energy eigenvalues in the absence of interaction, . The dressed and bare states are labeled beside the lines. denote the working frequency range of the quantum heat engine.

Ii The cQED System

We consider a single qubit, which could be either an atom or an artificial atom, trapped inside a high- single-mode resonator in a standard cavity QED or circuit QED geometry Walraff2004 (); Blais2004 (). In the absence of dissipation and driving and under the rotating wave approximation it is described by the Jaynes-Cummings Hamiltonian

(1)

with eigenstates

(2)

and eigenenergies

(3)

Here and are the excited and ground state of the qubit, with energy separation , are Fock states of the field mode of frequency , are Pauli matrices, and are bosonic annihilation and creation operators, is the vacuum Rabi frequency, is the qubit-field detuning, is the quantized generalized Rabi frequency

(4)

and

(5)

Fig. 1 shows the first few eigenenergies, illustrating the avoided crossing resulting from the dipole coupling between the qubit and the field at . Importantly for our discussion, the dressed states (qubit-photon polaritons), are photon-like for large positive detunings and qubit-like for large negative detunings, and the opposite for the dressed states .

The qubit and optical mode are also coupled to thermal reservoirs at temperatures and , respectively. In the following we consider the situation where and , a situation that would be characteristic of qubits confined in a cryogenic environment typical of circuit QED experiments and driven by a feeble thermal microwave field. The qubit-field system density operator is therefore governed by the master equation

(6)

where the Lindblad superoperators are , is the cavity mode decay rate, the qubit spontaneous decay rate, and the mean number of thermal photons within the resonator bandwidth.

Iii Heat engine

The difference in temperatures of thermal reservoirs for the qubit and the photon field allows one to operate a quantum Otto cycle. The following section discusses the operation of a single atom-single photon heat engine that exploits that cycle by varying the detuning .

iii.1 Single-photon case

The lowest state of the qubit-field system corresponds to the vacuum field state and is therefore qubit-like. The simplest way to operate the qubit-photon heat engine is to limit its operation to the ground state and the lowest energy dressed state (lowest polariton branch) . By varying the detuning from a negative to a positive value that state changes its nature from qubit-like to photon-like, thereby changing the thermal coupling from being to a bath at temperature to a bath at . Ideally, in the polariton picture the engine is then effectively a two-state system, while in the bare-mode picture it actually consist of two coupled qubits like the quantum engine proposed in Ref. Linden2010 ().

The operation of the engine relies on a four-stroke quantum Otto cycle Quan2007 (). The starting point of the cycle is the ground state with transition frequency and corresponding detuning , in thermal equilibrium at the qubit reservoir temperature . The first, isentropic stroke consists of changing to a new value and detuning . This step can be carried out relatively fast since it does not involve the approach of an avoided crossing where nonadiabatic transitions could be an issue. The second, isochoric stroke is the thermalization of the system with the two thermal reservoirs. Since nothing much happens to the qubit constituent of the system, but the field part acquires a finite probability to be excited to Fock states with For thermal microwave fields in the 100 GHz range and at temperatures around 1 K the only state that becomes significantly populated is the Fock state , with small probability . At the end of that step the qubit-field system is then left to a good approximation in the mixed state

(7)

The ground state component of plays no active role in the following third, isentropic stroke, so we concentrate of the state for now. In that stroke is changed back to its initial value , and the nature of the dressed state changes adiabatically from its approximate photon-like nature, , to its qubit-like form . This step must be carried out slowly enough that nonadiabatic transitions between the dressed states and remain negligible at the avoided crossing. Finally the last stroke is the spontaneous decay of the qubit-like state to the ground state at rate .

The thermalization strokes 2 and 4 are isochoric. Ideally no work is performed on the control field used to change during stroke 1 either, due to the vanishing population on the excited state . The only work contribution occurs during stroke 3, a result of the reduction in energy of the excited state population. The average work associated with a full Otto cycle is therefore

(8)

It is always negative, i.e. work is produced by the engine. Noting that and we have

(9)

We note for completeness that this system can also be operated as a heat pump, provided that , and that the cycle is reversed, with the initial state associated with a positive detuning , which is then changed to a negative value in the first stroke. The thermalization of the qubit at leads then to a population on the state . After an adiabatic change of the detuning back to a positive value the photon-like polariton decays back to the ground state at rate . In that mode of operation the average work is equal to which is positive, indicating that work is done on the system. This shows that in case the qubit thermalization dominates the system can operate as a heat pump, but if the thermalization of the field dominates it is a heat engine.

iii.2 Multi-photon case

For only the lowest polariton branch and the ground state are involved in the Otto cycle. In that limit the engine operation is formally identical with that of the optomechanical heat engine Zhang2014a (). For larger , however, higher polariton branches come into play. Specifically, at the end of the thermalization stroke the branches with are populated with thermal probabilities where is the average photon number. The result is the appearance of the superposition of several Otto cycles. The average work output produced in stroke 3 by the cycle associated with the polariton mode is

(10)

Following the thermalization stroke 4 the dressed state has relaxed to , . But in contrast to the situation for the polariton which is thermalized to the ground state , the first stroke of the next cycle now costs work. For the symmetric case and perfect adiabaticity that work is precisely equal to the work output of stroke 3 of the previous cycle, and the cycles associated with higher polaritonic modes produce no net work. As shown below the situation is slightly more favorable for the asymmetric situation , in which case some additional work can be extracted from the engine. For the opposite case , in contrast, stroke 1 costs more work than extracted during stroke 3.

As illustrated in Fig. 1, during the second, isochoric stroke of the engine, the dressed state is approximately identical with the bare state while provided that . Then at the end of the stroke, owing to the thermalization by an effectively zero-temperature qubit reservoir and a hot microwave reservoir, the state is essentially empty, while the ground state and the state are populated with an approximate microwave thermal distribution, resulting in an average energy

(11)

where and is the mean thermal photon number of the microwave field. During the third, isentropic stroke, is adiabatically changed back to . Then the dressed states and approach qubit-excited states and photon-excited states , respectively, with their population unchanged, so the average energy at the end is

(12)

The cooling of the heat engine takes place in the fourth, isochoric stroke by coupling it to the qubit reservoir at . During that stroke the heating from the microwave reservoir remains negligible for . This results in the transfer of population from the states to states , resulting in the occupation of dressed states . At the end of that stroke the average energy of the system is therefore

(13)

Finally, during the following isentropic stroke that brings the qubit frequency back from to the mean energy becomes

(14)

The work output is therefore

(15)

where the sum increases with the raising of temperature with the upper limit for . The maximum work output is therefore equal to the difference between the energy of a single photon and a single qubit,

(16)

The work input, on the other hand, is

(17)

So the total work reads

from which we can find that if and are chosen to be symmetrically detuned from , , the last term in Eq. (III.2) vanishes and the total work is precisely equal to the work output in the case of low-temperature microwave reservoir (see Eq. (9)). This is because except for the lowest two dressed states and , the work output and input arisen from the population of the higher dressed states cancel out each other in the Otto cycle, attributing to the symmetric structure of the energy spectrum of the states and . Then the total work reaches its maximum value at the precise temperature such that and . It then decreases is raised past that point.

There is however nothing fundamental about this result. This upper limit can easily be broken when the condition is no longer imposed. Specifically, for the last term becomes negative so the total work increases (the work output is negative, corresponding to an energy produce by the heat engine), while for the opposite case , the total work decreases.

Finally we note the unique role of in the work performed of the engine. Interestingly, this implies that for some non-equilibrium quantum reservoirs with lowered probability , e.g., a squeezed vacuum reservoir with , the total work can be significantly reduced, see Eq. (III.2).

iii.3 Two-qubit case

One can gain some intuition on the origin of the work generated by the engine by observing that provided there is at most one photon in the system the average work is independent of the number of qubits. Consider for concreteness the case of two qubits.

Figure 2: Dressed states picture for the two-qubit case. See the text for the definitions of the states and . Other parameters as in Fig. 1.

The total qubit-field Hamiltonian is then

(19)

where we have introduced the collective spin operators , . Much like for a single qubit, the Hamiltonian can be decomposed into invariant subspaces with excitations. The subspace is characterized by the ground state , and the one excitation subspace spanned by the two dressed states Wang2006 ()

(20)
(21)

Here

(22)
(23)
(24)
(25)
(26)

The corresponding energies are

(27)

with energy gap at the avoided crossing between and increased to , see Fig. 2. Then for an Otto cycle involving the same sequence of strokes as in the single-qubit case the average work is

(28)

which is same as Eq. (8) with replaced by , and is again bounded by Eq. (9). Having more than one qubit but only one photon doesn’t allow one to extract more work from the heat engine, demonstrating that it originates from the photon field. The generalization to qubits is straightforward, with the energy gap at the avoided crossing increasing to . This larger gap relaxes the time constraints associated with suppression of non-adiabatic transitions.

Iv Experimental considerations

In the following sections we focus for concreteness on the simplest case of a single qubit coupled to a single photon. Maintaining quantum adiabaticity in the isentropic stroke requires that changes in the qubit frequency should be slow enough to avoid transitions to the dressed state , yet faster than the qubit and cavity field decays. Also, must be much larger than to guarantee a full photon-like to qubit-like conversion of the nature of the polariton, but the detuning must remain sufficiently small, , for the rotating wave approximation and two-level approximation implicit in the Jaynes-Cummings Hamiltonian to remain valid. Turning to the two isochoric thermalization strokes, we note that stroke 2 only necessitates a time long compared to , while stroke 4 needs to occur in a time long compared to but short compared to to avoid a significant excitation of . Denoting the duration of the stoke as the hierarchies of system parameters required for the operation of the heat engine are therefore

(29)
(30)

Although these conditions are challenging for traditional cavity QED experiments, they should be realizable in circuit QED devices Schmidt2013 (). For a resonator frequency GHz Sandberg2009 () the mean photon number for a thermal blackbody spectrum at K is about , the single photon probability , and the occupation probability of the state is a negligible . The photon decay rate of the resonator and the qubit decay rate can be about kHz and MHz, respectively Underwood2012 (), and the dipole coupling frequency can be as high as MHz Peropadre2010 (); Hoffman2011 (), which leaves sufficient time for the adiabatic strokes.

A specific experimental design of the engine that permits to extract work in an exploitable form, we consider a superconducting transmon qubit. Its frequency can be adjusted by controlling the magnetic flux , with  Majer2007 (). In the bare-mode picture the quantum expression for the infinitesimal average work is

(31)

Because is an implicit function of the magnetic field intensity Eq. (31) is equivalent to . This suggests that the engine can be treated as an artificial magnetic substance with effective average magnetic moment located in a circuit loop. In stroke , besides adjusting , the change in also induces a current in the circuit according to Faraday’s law, but no work is done by the magnetic substance since and . However in the third stroke so that even when applying an equal change in the induced current is different. The work outputed by the magnetic substance, i.e. the engine, is responsible for the increase in current, which could be further extracted via coupling to additional elements.

V Work measurement

A straightforward two-point energy measurement based on Eq. (8) is unsuitable to measure the work of the polariton engine since polaritons are quasiparticles that cannot be directly detected Dong2015 (). The integral from to of Eq. (31) provides an equivalent expression for the work and suggests that the average work and its fluctuations can be measured by monitoring . However, as should be expected the statistical properties of the measured work depend on the measurement protocol, since different schemes result in general in different measurement backaction. We now compare the results obtained from two different types of measurement.

v.1 Dispersive quantum measurements

If we use a secondary probe beam dispersively coupled to the qubit by the interaction

(32)

where and are the annihilation and creation operators of the probe Blais2004 (), then the repeated homodyne detection of the probe provides a sequence of measurements of .

Ignoring for now effects due to dissipation during the work-producing isentropic stroke , the time evolution of the system is described by the stochastic Schrödinger equation Jacobs2006 (); Gambetta2008 (); Zhang2011 ()

(33)

where characterizes the measurement strength and is an infinitesimal Wiener increment. Repeatedly solving Eq. (33) with the initial state (7) and a slowly-varied generates a set of quantum trajectories . The mean and variance of the work, as well as the back-action of the measurements are readily obtained from the statistical properties of these trajectories Horowitz2012 (); Hekking2013 (). This also means that the statistics of the work depends on the quantum measurement schemes.

Figure 3: Upper plot: Dressed states and bare states population dynamics during the isentropic stroke 3 in the absence of measurements (), and for measurement strengths and . Here the qubit frequency varies linearly in time from to and . Lower plot: Log scale probability distribution of the measured work obtained from 1000 stochastic quantum trajectories for the same measurement strengths.

Fig. 3 summarizes the results of simulations for a set of parameters within state-of-the-art experimental reach. The upper part of the figure plots the evolution of the average populations of the relevant states of the qubit-field system during the third stroke of the cycle, and the lower part shows the probability distribution of the work extracted in a single cycle of the engine in the absence of measurements and for two measurement strengths .

In the absence of measurements the bare states and exchange their populations almost perfectly as is decreased slowly from to across the avoided crossing. The occupation probability of the dressed state remains nearly unchanged, confirming the almost perfect adiabatic conversion of the polariton from photon-like to qubit-like. As expected is a double-peaked distribution with taking the value with probability and with probability . That latter dominant component footnote2 () is due to the population of the state , which is not involved into the heat engine cycle.

Because the dispersive coupling of the qubit to the probe field does not commute with the Jaynes-Cummings Hamiltonian (1) it couples the two dressed states and and with an imperfect conversion between the two bare states and . This results in a measurement back-action whereby the peak in at broadens and spreads towards the zero, as visible in the upper part of Fig. 3. As increases the adiabatic conversion gradually breaks down and the populations of states and approach equal values, with the system evolving toward the deterministic steady-state

(34)

with a significantly reduced average work.

In addition to measurement-induced dissipation, the effects of qubit and cavity dissipation on the average work during the isentropic stroke can be evaluated quantitatively by solving Eq. (6). Physically, the spontaneous decay of the qubit from to is dominant for , and results in a reduction of the average work. For the thermalization of the cavity mode causes transitions from to , increasing the work produced by the QHE. In contrast, for it induces transitions from to , whose population then transfers to the state during the thermalization stroke , thereby opening up a leak in the Otto cycle. That leak is minimized by imposing .

v.2 Absorptive quantum measurements

Figure 4: Same plots as Fig. 3 but for the resonant absorptive measurement.

To illustrate the dependence of the statistical properties of the measured work on the measurement protocol we compare the homodyne detection with large-detuned probe to a resonant absorption measurement scheme. This can be realized by resonantly coupling a low-density ground state beam of probe two-state systems with the qubit through the interaction

(35)

where the superscripts “” labels the spin operators of the probe qubits. Ignoring the effects of dissipation during the adiabatic stroke 3 (same as in the dispersive case), the time evolution of the system is then described by the stochastic Schrödinger equation Jacobs2006 (),

(36)

where is a measure of the strength of the measurement and is an infinitesimal Ito increment. The results of simulations are shown in Fig. 4 with all parameters as in Fig. 3. In the absence of measurements the evolution of the population of the relevant states and the statistics of the work output are the same in the two figures, as should of course be the case, but as the strength of the measurement increased, the populations of the states and now decay to zero and the populations of the states and remain equal to zero in the end of stroke 3. This is attributed to the absorption from the probe, which results in a measurement-induced energy loss. As a result the average work decreases dramatically, with an associated broadening of the distribution of towards zero.

Vi Conclusion

To summarize, we have proposed and analyzed what is arguably the simplest polaritonic QHE, a single qubit coupled to a single photon that operates by absorbing energy from feeble thermal microwave fields. Irrespective of its experimental implementation it offers a straightforward and pedagogically appealing platform for quantitative studies of quantum thermodynamics. Circuit QED realizations of this system seem particularly promising, in which case the work output is readily controllable and extractable, and the influence of the quantum measurement can be demonstrated efficiently.

Vii Acknowledges

We acknowledge enlightening discussions with K. Schwab, A. Kamal and L. Zhou. This work is supported by National Key Research and Development Program of China No. 2016YFA0302000. QS and KZ are supported by NSFC Grants No. 11574086, 91436211, 11654005, and the Shanghai Rising-Star Program 16QA1401600. SS and PM are supported by the U.S. Army Research Office. WZ is supported by NSFC Grant No. 11234003.

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