Effective spin-chain model for strongly interacting one-dimensional atomic gases with an arbitrary spin

Effective spin-chain model for strongly interacting one-dimensional atomic gases with an arbitrary spin

Lijun Yang and Xiaoling Cui xlcui@iphy.ac.cn Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing, 100190, People’s Republic of China
July 5, 2019
Abstract

We present a general form of the effective spin-chain model for strongly interacting atomic gases with an arbitrary spin in the one-dimensional(1D) traps. In particular, for high-spin systems the atoms can collide in multiple scattering channels, and we find that the resulted form of spin-chain model generically follows the same structure as that of the interaction potentials. This is a unified form working for any spin, statistics (Bose or Fermi) and confinement potentials. We adopt the spin-chain model to reveal both the ferromagnetic(FM) and anti-ferromagnetic(AFM) magnetic orders for strongly interacting spin-1 bosons in 1D traps. We further show that by adding the spin-orbit coupling, the FM/AFM orders can be gradually destroyed and eventually the ground state exhibits universal spin structure and contacts that are independent of the strength of spin-orbit coupling.

I Introduction

Strongly interacting system is known to be notoriously difficult to solve in physics. There is one exception, however, for the infinite coupling of one-dimensional (1D) system that the exact solutions of bosons and fermions can be constructed taking advantage of the peculiar feature of femionalizationGirardeau1 (); Girardeau2 (); Sengstock (); Chen (); Girardeau3 (). In cold atoms experiments, strongly interacting Tonks-Girardeau gases have been realized in both spinless bosonsBloch (); Weiss (); Haller () and spin-1/2 fermionsJochim1 (); Jochim2 (); Jochim3 (). A fascinating property with an infinite coupling (hard-core interaction) is that, the ground states of a spinful system are highly degenerate and their wave functions share the form of

(1)

Here and are position and spin of the -th particle ; is the Slater determinant made up of the lowest N-level of eigenstates in 1D system, a common factor of all degenerate wave functions . While the energy of is solely given by , the part uniquely describes the distribution of spins in the coordinate space and determines the degeneracy of the system. The large degeneracy has been shown to facilitate the Ferromagnetic transition of spin-1/2 fermions as tuning the coupling strength across this critical pointCui1 (); Cui2 ().

Apart from the infinite coupling case, it is interesting and also more practical to learn about the physics in the regime of large but finite couplings. This regime is more realistic to achieve in experiments, which can be adiabatically connected to the non-interacting limit as tuning the interaction strength. With finite couplings, the magnetic properties of bosons and fermions are very different. General theorems have shown that the ground state for spin-1/2 fermions is with the lowest total spinLieb-Mattis (), while for iso-spin 1/2 bosons is ferromagneticFM1 (); FM2 (); FM3 (). Accordingly, the effective anti-ferromagnetic(AFM) and ferromagnetic(FM) spin-spin exchange interactions have been successfully extracted from the Bethe-ansatz solutions of strongly coupling spin-1/2 fermionsGuan_f () and bosonsGuan_b (). Recently, taking advantage of the high controllability of a few particles in the trapped ultra-cold systemsJochim_expe (), a number of studies have revealed the energy spectra and correlation effects for a few spin-1/2 fermions by numerical simulationsBlume (); Conduit (); Lewenstein (); Zinner1 (). In the strong coupling regime, an effective Heisenberg spin-chain model has also been deducedZinner2 (); Santos (); Pu (); Levinsen (). The resulted anti-ferromagnetic correlation has recently been confirmed through the tunneling measurement of a few spin-1/2 fermions in 1D trapsJochim_chain (). Moreover, the effective models for spin-1/2 bosonsZinner3 (); Levinsen2 () and for higher-spin case with SU(N) symmetryZinner2 (); Santos () have also been discussed.

In this work, we will present a general form of the effective spin-chain model for strongly interacting trapped atomic gases with an arbitrary spin and arbitrary statistics (Bose or Fermi). In particular, for high-spin atomic systems, the multi-channel interactions can break the SU(N) symmetry and the ground state can have a wide variety of magnetic orders, including FM, AFM or even intriguing ones, depending on the relative coupling strength between different scattering channels. We find that the resulted form of effective spin-chain model generically follows the same structure as that of the interaction potentials classified by scattering channels, thus respects the symmetry of original Hamiltonian for trapped systems. This form can be applied to any spin-value, Bose or Fermi statistics and confinement potentials. Take the strongly interacting spin-1 bosons for example, we adopt the effective spin-chain model and reveal both FM and AFM correlations by choosing different interaction strengths for different cold atoms.

Based on the spin-chain model, we further study the effect of spin-orbit coupling(SOC), which has been realized in cold atoms experiments by the two-photon Raman processesIan_1 (); Ian_2 (); Shuai (); Jing (); Martin (); Engels (). For spin-1 bosons, we will show how the FM or AFM correlations being destroyed as increasing the SOC strength. In the SOC-dominated regime, we obtain universal spin texture and contacts, which are independent of the actual SOC strength. These results are consistent with previous studies on the spin-orbit coupled spin-1/2 fermions at infinite coupling Cui3 (); Blume2 ().

The rest of the paper is organized as follows. In section II, we present the derivation of the effective spin-chain model with an arbitrary spin. We will first take the spin-1/2 (two-component) fermions and bosons as a starting point, to get insight to the general structure of spin-chain models with an arbitrary spin. In section III, based on the effective spin-chain model, we study the system of spin-1 bosons and show the ground state exhibiting FM or AFM correlations. We further study the interplay effect of strong interaction and SOC to the ground state properties of spin-1 bosons under the effective spin-chain model. Finally we summarize in section IV.

Ii Effective spin-chain model

We first write down the non-interacting Hamiltonian for atoms confined in the 1D trap,

(2)

Here is a spin-independent trapping potential and in this paper we consider a harmonic trap with trapping frequency and characteristic length . The interaction is generally characterized by the coupling constant , and for the high-spin atoms there can be multiple scattering channels with multiple coupling constants. In this work we consider the large repulsive coupling constants in all scattering channels, which can be achieved through the confinement induced resonanceOlshanii () or the preparation of very dilute gas.

The basic idea for the construction of an effective spin-chain model is that, the physics in the vicinity of infinite coupling can be well deduced from the known limit, by treating as a small parameter in the framework of the perturbation theory. In this way the wave function to the zeroth order of can be approximated as certain superposition of the degenerate states at , which leads to an energy functional up to the linear and gives the effective model. This idea has been successfully applied to the spin-1/2 fermion case and leads to the AFM Heisenberg spin-chain model thereinZinner2 (); Santos (); Pu (); Levinsen ().

In this section, we will first give a detailed introduction to the degenerate ground states at infinite coupling, as they are essential for the construction of spin-chain model when slightly away from this special point. These degenerate states are classified by the order of spins in coordinate space and thus named as the spin-ordered states as in Ref.Cui3 (). Using these states, we will re-derive the spin-chain model for the spin-1/2 fermions and bosons as a starting point. Finally, we will extend our derivation to an arbitrary spin case and present a general form of spin-chain model for both fermions and bosons.

ii.1 Spin-ordered state

To conveniently enumerate the degenerate ground states at infinite coupling of 1D systems, we define the spin-ordered state:

(3)

In this state, a sequence of spins , is placed in order in the 1D coordinate space. Explicitly, its wave function is written as

(4)

where is a permutation of the integers , and

(5)

The spin-ordered state as defined in (3) is symmetric under the simultaneous change of the coordinate and spin of any two particles. It is then straightforward to construct the degenerate ground states of bosons and fermions at infinite coupling using this class of states:

(6)
(7)

here () is the wave function of bosons (fermions) obeying Bose (Fermi) statistics; is the Slater determinant composed by the lowest N-level of eigenstates of in Eq.2:

(8)

with a fully symmetric function (with respect to the exchange of any two coordinates). In Eqs.(6,7), the part determines the ground state energy of the system, while the part uniquely determines the spin distribution/order of system. By considering different spin orders in , one can cover all the degenerate ground states at infinite coupling. Moreover, it is easy to check that the states with different spin orders are orthogonal to each other. Therefore, the wave functions as Eqs.(6,7) constitute a complete and orthogonal set of basis in ground state manifold of particles with infinite coupling strength.

Given Eqs.(6,7), one can compute the particle density at the th spin order:

(9)

with . gives the probability of finding the th ordered particle at position and we have . In Fig.1, we show (with ) for particles in a 1D harmonic trap. It is found that the density peak for each spin order is well separated from each other, and can be well approximated by a Gaussian functionCui3 ():

(10)

here is the averaged location of the th particle, and is the width of the density distribution for the th particle which can be obtained by fitting with above function. In Table I, we present the result of , and for particles. It is found that the neighboring and are nearly equally spaced by a distance , and each is typically of order of and varies little for different .

Figure 1: (Color online). The particle density (blue dashed lines) for particles in a harmonic trap. and are respectively in the unit of and , with the confinement length of the trapping potential. The black curve shows the total density . Here the spin-order index is mapped to the site index in the effective spin-chain model.
1 2 3 4
-1.751 -0.551 0.551 1.751
1.200 1.102 1.200 -
0.739 0.653 0.653 0.739

1 2 3 4 5 6
-2.451 -1.466 -0.450 0.450 1.466 2.451
0.985 1.016 0.900 1.016 0.985 -
0.684 0.595 0.567 0.567 0.595 0.684

1 2 3 4 5 6 7 8
-3.049 -2.044 -1.189 -0.394 0.394 1.189 2.044 3.049
1.005 0.855 0.795 0.780 0.795 0.855 1.005 -
0.648 0.556 0.522 0.508 0.508 0.522 0.556 0.648
Table 1: The averaged location , the difference and variance for .

When limited to the ground state manifold, we can map the spin-order index to the site index , and thus the physics with spin-ordered state can be mapped to that under an effective spin-chain model. Here we like to point out an essential difference between the effective spin-chain and the real lattice configuration, that the particle density at each ”site” of the effective spin-chain can actually spread over the inter-particle spacing of atoms in the harmon trapnote_density (), while in the real lattice case just localize around each lattice site. The large spreading in the effective spin-chain case can lead to strong interference of spins between neighboring orders and give rise to exotic spin density profiles Cui3 ().

ii.2 Effective spin chain model for spin-1/2

In this section, we will derive the spin-chain model for spin-1/2 system, which was previously studied in Ref.Zinner2 (); Santos (); Pu (); Levinsen (); Zinner3 (); Levinsen2 (). Here we will adopt a systematic method in order for easy generalization to the high-spin case.

For spin-1/2 system with total particle number , the number of different spin-ordered states, i.e., the ground state degeneracy at infinite coupling, is .

ii.2.1 spin-1/2 fermions

Due to Fermi statistics, the contact interaction for spin-1/2 fermions only occurs in the spin-singlet channel with coupling constant . In fact, in this case one can directly write the interaction as

(11)

because the particles scattering in other channels (other than spin-singlet) will be automatically ruled out by the asymmetric feature of the wave function (or the Fermi statistics).

For large (and thus small ), the many-body wave function can be written as certain superposition of the degenerate ground states (Eq.7) at :

(12)

At small , the associated energy can be expanded as:

(13)

where is the degenerate energy at (determined by ), and is proportional to the Tan’s contact in 1DContact_1D ():

(14)

In the following, we will aim at expressing in terms of the coefficients in Eq.(12), which is essential to the construction of effective spin-chain model.

Applying the Hellmann-Feynman theorem HF () to Eq.(14), we obtain

The integral in above equation can be obtained by considering the Schrodinger equation:

with respectively represent the relative and center-of-mass motions of and particles. The boundary condition around gives

(17)

So we get in Eq.(II.2.1) as

(18)

Given the property of in Eq.(8), can be further reduced to:

Due to the inclusion of , it is easy to check that only when the two coordinates, and , stay in the neighboring order in the wave function, can they have contribution to . Assume and stay in the th and th order in , we denote their contribution to as . For two particles there are four spin-ordered states:

(20)

and they can form one singlet and three triplets:

According to the definition of spin-ordered states in Eq.(4), above states can be simplified as:

It is then easy to see that only the singlet state, , can contribute to in Eq.(II.2.1). Physically, this is due to the Fermi statistics and the asymmetric feature of the fermionic wave function (12).

As the spin-ordered states in the wave function (12) can be classified according to the total spin and total magnetization of the -th and -th ordered particles, we can write

(21)

here can be ; means the spin-ordered states for the other order numbers except and . Based on (21), we can obtain as:

(22)

here is at the -th order in the -function (i.e., there are number of particles with coordinates smaller than ). The contribution of these two order numbers ( and ) to the energy (13) is (up to a constant ):

(23)

Now we go on to construct an effective spin-chain model, by replacing the spin-order index with the lattice site index in Eq.(21). In order to obtain the same energy functional as (23), the only way is to consider the following effective Hamiltonian

(24)

with the projection operator for neighboring sites ( and ) forming a singlet, and follows

By expanding in terms of the Pauli matrix and also noting that the total Hamiltonian is the summation of all neighboring-pair contributions, , finally we arrive at the effective spin-chain model for spin-1/2 fermions:

(26)

The result of anti-ferromagnetic correlation in above Hamiltonian is consistent with the Lieb-Mattis theorem saying that the ground state of spin 1/2 fermions is with the lowest total spinLieb-Mattis (), as well as the indication from Bethe-ansatz solutionsGuan_f ().


ii.2.2 spin-1/2 bosons

For two-component (with pseudo-spin ) bosons, the interaction can occur in three channels:

(27)

These channels actually represent three spin-triplet channels due to the Bose statistics.

For large , the many-body wave function can be written as certain superposition of the degenerate ground states (Eq.(7)) at all :

(28)

here the wave function is distinct from Eq.(12) by replacing with its absolute value. This replacement will significantly affect the expression of as defined in the energy expansion at small :

(29)

with given by:

(30)

Following the similar procedure as in the last section, we obtain as:

(31)
(32)
(33)

Again we select out two coordinates, and , staying in the neighboring orders, -th and -th, in the wave function, and denote their contribution to as . After simple algebra, we find that only the three triplet can contribute; explicitly, and respectively contribute to and . By rewriting the spin-ordered state as the form of Eq.(21), we can then obtain

(34)
(35)
(36)

here follows the same expression as Eq.(LABEL:J_l). Considering the energy functional (29), and replacing the spin-ordered index in (21) as the lattice site index, we can write down the effective spin chain model as

(37)

with the projection operator for neighboring sites and forming a triplet with . For the case of , Eq.(37) can be reduced to the XXZ Heisenberg model:

(38)

For the case of interaction with spin-independent interaction strength , Eq.(37) is reduced to the isotropic Ferromagnetic Heisenberg model:

(39)

This is consistent with general theorems showing that the ground state of iso-spin 1/2 bosons is ferromagneticFM1 (); FM2 (); FM3 () and with the result from Bethe-ansatz solutionsGuan_b (). We note that the effective models (Eqs.38,39) preserve the full symmetry of original Hamiltonian, as they take the same structure as that of the interaction potentials. These models are related to those in Ref.Zinner3 (); Levinsen2 () by a unitary transformation with operator note_boson_model ().

Comparing spin-1/2 bosons with fermions, we can see that the distinct correlations (FM for bosons and AFM for fermions) in Heisenberg Hamiltonians are intrinsically resulted from the different symmetries allowed for the system. For the fermions, the anti-symmetric feature of the wave function requires that the particles scatter in the singlet channel, while for bosons the symmetric wave function requires the triplet channels. These scattering channels uniquely determine the structure of the effective models (see Eqs.(24,37)) in terms of the projector operators . This structure manifests the intrinsic relation between the statistics, the interaction channels, the effective spin-chain Hamiltonian and the nature of the ground state. In the following, we will show that it can be straightforwardly generalized to an arbitrary high-spin case.

ii.3 Effective spin-chain model for a general spin

For a general high-spin system with multi-channel scatterings, the interaction can be written as :

(40)

Here is the coupling constant for two particles scattering with total spin and total magnetization ; is the projection operator for particles scattering in the sector.

For large , the many-body wave function of bosons (B) and fermions (F) can be respectively written as:

(41)
(42)

The energy expansion at small can be expanded as:

(43)

with given by:

(44)

The boundary condition around gives

(45)

with the many-body wave function for bosons or fermions. Based on this boundary condition, we can expand (44) as

(46)

for fermions, and

(47)

for bosons. Assume two coordinates, and , staying in the neighboring orders, -th and -th, in the wave function, and denote their contribution to as . Due to the sign difference in the expressions of for bosons and fermions, we find that only when the spin wave function in the spin-ordered states is symmetric for bosons and antisymmetric for fermions, can it contribute to . This can also select out the spin channels in which the particles can scatter with each other.

By rewriting the spin-ordered state as the form of Eq.(21), we can obtain

(48)

here follows the same expression as Eq.(LABEL:J_l). Considering the energy functional (43), and replacing the spin-ordered index in (21) as the lattice site index, we can write down the effective spin chain model as

(49)

with the projection operator for neighboring sites and forming a state with total spin and total magnetization . Above results can be easily applied to the spin-1/2 case of fermions () and bosons (), and accordingly the AFM or FM Heisenberg models can be obtained respectively.

To this end, we have obtained a general form of effective spin-chain model, Eq.(49), to describe strongly coupling atoms in 1D trapped system. It can be applied for any statistics (Bose or Fermi), an arbitrary spin, and any spin-independent confinement potential. A key property of this effective model is that locally for each site the Hamiltonian can be well separated into two parts: the coupling parameter which only relies on the local scattering amplitude, and the nearest-neighbor spin-projection which follows the same structure as the interaction model. This is closely related to the spin-charge separation in the wave function in the hard-core limit, as the form of Eqs.(41,42). More explicitly, the charge part () determines the local scattering amplitude , while the spin-ordered part together with the statistics determine the spin-relevant terms in Eq.(49).

Iii Strongly coupling spin-1 bosons and the effect of spin-orbit coupling

In this section, we will apply the effective spin-chain model (49) to the spin-1 bosons. At low fields, the interaction of spin-1 bosons has symmetry and can be classified into two channels:

(50)

here and are respectively the coupling constant in the total spin and channelsspin1_H_1 (); spin1_H_2 (), and is the projection operator to the total spin -channel. Depending on the relative strength of and , the cold atoms system can have AFM (or polar/nematic) ground state (Na with ), or FM ground state (Rb with ).

Based on the general formula (49), we can obtain the effective spin-chain model for spin-1 bosons in the strong coupling limit:

which can be reduced to the form:

with the spin operator at site . In writing above equation, has been decomposed as the product of and . is a quantity that only depends on the total particle number and the underlying trapping potential, which is proportional to the contact of the system, while the site-dependence of is simply included in . Since does not depend on the spin, here we use a good approximation derived for the spin-1/2 fermions case in a harmonic trapLevinsen ():

(53)

in Eq.III are dimensionless parameters depending on the ratio of interaction strengths in different channels:

(54)
(55)
(56)

Note that the structure of the Hamiltonian (III) is the same as that of the bilinear-biquadratic isotropic quantum chain and that in the Mott phase of spin-1 bosons in optical lattices spin1_1 (); spin1_2 (); spin1_3 (). The only difference is that here the coupling constants of neighbor spins are site-dependence, due to the background trap potential and the resultant inhomogeneous particle (charge) density.

When add the spin-orbit coupling(SOC) to the system, which corresponds to a rotating field in the coordinate spaceIan_1 (); Ian_2 (); Shuai (); Jing (); Martin (); Engels ():

the spin texture and the spin-spin correlation according to (Eq.III) can be greatly modified. In the basis of spin-ordered states, the SOC Hamiltonian can be greatly reduced similarly to the spin-1/2 fermion caseCui3 ():

(58)

Here and Cui3 (), with the averaged defined in Eq.10 and the mean particle distance . We make such approximation by noting that and differ little between different , as shown in Table I. Moreover, here as we are limited at small and moderate , we have neglected the contribution from higher harmonic levels and thus the extra spin-exchange terms as pointed out in Ref.Blume2 ().

Figure 2: (Color online). Energy spectrum as a function of spin-orbit coupling strength for Na (a) andRb (b) atoms with total number . is chosen to be . All energies are in the unit of . Different colors represent different spin values determined by .

In Fig.2, we show the energy spectrum as a function of for both Na () and Rb () systems with particle number and rotation angle . In the absence of SOC (), the total spin is conserved. For Na, the ground state is a singlet with , and as increases the energy also increases. For Rb, the situation is reversed: the ground state is highly degenerate with the largest total spin , and the energy increases as decreases. For both Na and Rb, we can see that the states are degenerate for different magnetization with the same . However, this is no longer true when turn on even a tiny strength of SOC (). In this case, the original degeneracies are completely lifted, as shown by Fig.2(a,b), because the SOC field in (58) does not commutate with the total spin.

Figure 3: (Color online). The ground state energy (a) and total spin (b) as a function of for both Na and Rb. All parameters are the same as in Fig.2. Gray dashed line in (b) shows the universal value in the SOC dominated regime.

In Fig.3, we show the ground state energy and as a function of . We see that of both Na and Rb decrease as increasing , while the total spin tend to approach the same value at . In this regime, the AFM or FM correlation in the spin chain model is fully destroyed by the SOC field, and the systems of both Na and Rb are fully governed by the local rotating field in (Eq.(58)). Thus increasing , the system will undergo a crossover from the interaction-dominated to the SOC-dominated regime.

Figure 4: (Color online). Local spin in the ground state at several values of for Na (upper panel) and Rb (lower panel) atoms. All parameters are the same as in Fig.2.
Figure 5: (Color online). Spin-spin correlation in the ground state at several values of for Na (a) and Rb (b) atoms. All parameters are the same as in Fig.2. Gray dashed lines show the universal value in the SOC dominated regime.
Figure 6: (Color online). Contact (, in the unit of ) for the ground state as a function of for Na and Rb atoms. All parameters are the same as in Fig.2. Gray dashed lines show the universal values in the SOC dominated regime.
Figure 7: (Color online). The contacts (in the unit of , upper panel) and the total spin as functions of rotation angle (in the unit of ) for the ground states of particles in the SOC-dominated regime.

One can also see the evidence of such crossover by examining the spin structure and the contact of the system. Fig.4, Fig.5 and Fig.6 respectively show the spin texture , nearest-neighbor correlation , and the contacts () for the ground states of Na and Rb at several values of . At zero or small , we can see clearly the signature of AFM or FM correlations: for Na, for all characterizing the polar/nematic ground state; for Rb, we have for all , for any nearest-neighbor pair, and all characterizing a FM state. As increasing , both Na and Rb will develop a large spin spiral with amplitude of the order of unity (see Fig.4). Consequently, and also approach universal values for both Na and Rb which do not change as increasing further (see Fig.5 and Fig.6). When at the special point of infinite coupling, any infinitesimal will induce a large and universal spin-spiral, as identified previously in the spin-1/2 fermions case Cui3 ().

In the SOC-dominated regime, each site in the spin-chain model (III) is decoupled from others and the ground state can be straightforwardly obtained as

(59)

here is the creation operator of a single atom with magnetic number at site . Given the wave function (59), we can get the following universal physical quantities:

(60)
(61)