# Crossover between spin swapping and Hall effect in metallic systems

###### Abstract

We theoretically study the crossover between spin Hall effect and spin swapping, a recently predicted phenomenon that consists in the interchange between the current flow and its spin polarization directions [Lifshits and D’yakonov, Phys. Rev. Lett. 103, 186601 (2009)]. Using a tight-binding model with spin-orbit coupled disorder, spin Hall effect, spin relaxation and spin swapping are treated on equal footing. We demonstrate that spin Hall effect and spin swapping present very different dependences as a function of the spin-orbit coupling and disorder strengths. As a consequence, we show that spin swapping may even exceed spin Hall effect. Three set-ups are proposed for the experimental observation of the spin swapping effect in metals.

## I Introduction

The spin-orbit coupling (SOC) is a relativistic effect that couples the particle’s spin degree of freedom to its orbital angular momentum. In solid-state, this coupling originates from the interaction between the carrier’s spin and the magnetic field that it experiences in its rest frame in the presence of a potential gradient (crystal field, defects etc.). The locking between spin and orbital angular momenta has spectacular consequences in normal metals such as, but not limited to, spin Hall effect dyakonov-perel1971 (); kato_science2004 (); wunderlich_prl2005 (), spin galvanic effect ivchenko1989 (); ganichev2001 (); ganichev2002 () and spin relaxation dyakoperel (); fabian2007 (); wu2010 (). In semiconductorsdyakonov2008 (), metalsjungwirth2012 (); hoffman2013 (); sinova2014 () and more recently topological insulatorsHasan2010 (), SOC is now commonly engineered and exploited to generate pure spin currents, thereby enabling the electrical manipulation of the spin degree of freedom in the absence of an external magnetic field.

The most emblematic effect induced by SOC is probably the spin Hall effect (SHE) originally predicted by Dyakonov and Perel dyakonov-perel1971 () and revived thirty years later by Hirsch hirsch () and Zhang zhang2000 (). In analogy with the ordinary Hall effect, SHE consists in the generation of a transverse spin current in response to an electric field applied in the longitudinal direction. Geometrically, the spin current has the form , where is a spin current polarized along the direction and flowing along the direction , is the electric field applied along the direction , is the longitudinal conductivity, is the spin Hall angle (measured in %) and is Kronecker symbol. In their pioneering theory, Dyakonov and Perel derived SHE from Mott scattering on spin-orbit coupled impurities, i.e. from the asymmetric spin-dependent scattering of an initially unpolarized electron flow smit_1955 (); smit_1958 (). This mechanism is usually referred to as extrinsic since it depends upon the presence of impurities in the system. Another extrinsic effect that occurs upon scattering is the shift of the position of the incoming wave packet, called side jump scattering berger_1970 (). This shift renormalizes the velocity operator by creating an effective anomalous velocity proportional to the number of impurities in the system lyo1972 ().

Besides extrinsic contributions to SHE, the spin-orbit coupled band structure may also dramatically influence the velocity of traveling electron wave packets even in the absence of impurity scattering. Indeed the velocity operator, , is affected by the SOC present in the band structure which induces an additional Lorentz force that bends the trajectory of Bloch states karplus1954 (). The effective magnetic field felt by the moving electron (also called Berry curvatureberry (); berryphase ()) and arising from the band structure is intrinsic as it does not rely on impurity scattering. This contribution has been widely studied in the context of anomalous Hall effect Nagaosa2010 (), for instance. The first prediction of impurity-free intrinsic SHE in non-centrosymmetry semiconductors sinova2004 (); murakami_science2003 () paved the way towards the prediction and discovery of topological insulatorsHasan2010 ().

The search for efficient SHE has been quite intense in the past ten years jungwirth2012 (); hoffman2013 (); sinova2014 (). After its pioneering observation in semiconductors kato_science2004 (); wunderlich_prl2005 (), the attention has quickly drifted towards the exploration of metals valenzuela2006 (). A wide variety of noble and transition metals has been investigated and while the exact values and the proper method to detect SHE is still under debate, clear indication of intrinsic SHE Guo2008 (); tanaka2008 () has been established in 4 and 5 noble metals (Pt, Pd, Ta, W etc. - see Ref. vila2007, ; mihajlovic_prl2009, ; mosendz2010, ; morota2011, ; pai2012, ; fujiwara_nature2013, ), as well as in 3 transition metals du2014 (). Alternatively, it has been recently suggested that large spin Hall angle could be achieved by exploiting skew scattering on the resonant states of 5 or 4 impurities embedded in a light metal matrix, such as Cu or AlGuo2009 (); tanaka2009 (); fert2011 (); levy2013 (). Evidence of large Hall angles from resonant skew scattering was reported in Pt- seki_nature2008 (); gu2010 () and W-doped Au Laczkowski2014 (), as well as Ir- niimi_prl2011 () and Bi-doped Cu niimi_prl2012 ().

Metals doped with heavy impurities present an interesting paradigm as they may be utilized to observe novel effects such as spin swapping (SSW), i.e. the conversion of a spin current into a spin current upon scattering by spin-orbit coupled impuritieslifshits_prl2009 (); sadjina2012 (). In the present work, we explore the nature of spin-orbit coupled transport within a disordered tight-binding model and demonstrate the emergence of SSW when the injected current is spin-polarized. In our model, SSW, SHE and spin relaxation all arise from the same spin-orbit coupled disorder which allows us to treat these different effects on equal footing. In particular, a crossover between SSW and SHE, controlled by the spin relaxation, is revealed and analyzed. This article is organized as follows. The physics of impurity-induced spin swapping is first outlined in Section II. In Section III, a single band tight-binding model and the corresponding non-equilibrium Green’s function technique are presented. Section IV is devoted to the numerical results. Finally, Section V suggests three setups for the experimental observation of SSW, and Section VI concludes this study.

## Ii Physics of spin swapping

The physics of extrinsic Mott skew scattering and SSW is illustrated on Fig. 1(a) and (b), respectively. Let us first consider spin-dependent scattering against a spin-orbit coupled impurity. In real space, the impurity potential reads

(1) |

where is the spin-independent impurity potential, and is the SOC parameter of the impurity. In the reciprocal space, this impurity potential becomes

(2) |

It is clear that the spin-orbit coupled part of the impurity potential acts like a magnetic field on the incoming electron spin , where is the momentum of the incoming electron and is the momentum of the outgoing electron. Therefore, in the case of an unpolarized charge current, this magnetic field defines a local quantization axis so that one can phenomenologically separate electrons with a spin polarization pointing parallel and antiparallel to , as illustrated on Fig. 1(a). In this case, proper treatment of the collision integral leads to Mott scattering, i.e. electrons with a spin momentum pointing (anti)parallel to have the tendency to scatter towards the left (right). The resulting spin current is therefore polarized along and flows transversely to both and . This mechanism is at the core of the skew scattering mechanism giving rise to SHE as originally pointed out by Dyakonov and Perel dyakonov-perel1971 ().

Let us now consider an incoming spin-polarized current (it can be either a pure spin current or accompanied by a charge flow), whose spin polarization lies in the scattering plane (). In this case, the incoming spin precesses around the effective magnetic field . Since this magnetic field only exists upon scattering from to , the spin polarization of the outgoing current is re-oriented lifshits_prl2009 (). Lifshits and Dyakonov tagged this effect ”spin swapping” as the spin polarization and flow direction of the incoming spin current are swapped during this process: an incoming spin current gives rise to a spin current when (similarly a spin current, say, produces two spin currents and ).

Physically, SSW is nothing but a spin precession around the spin-orbit field . Such precessions are well known in semiconductors possessing Rashba, Dresselhaus or Kohn-Luttinger SOC dyakonov2008 (). This SOC-induced precession has been utilized in the Datta-Das transistor datta90 (); koo09 () (see also Ref. sadjina2012, ) and its impact on spin transfer torque has been investigated in (Ga,Mn)As-based spin-valves haney2010 () and single layers Li2015 (). However, the impurity-induced spin swapping presents a number of interesting differences. First, in contrast with coherent spin precession around Rashba or Dresselhaus SOC, spin swapping arises from spin precession stemming from incoherent scattering. It is quite remarkable that this effect survives the disorder configurational average, as does extrinsic SHE. A spin diffusion equation in the presence of spin-orbit coupled impurities within the first Born approximation has been derived by Shchelushkin and Brataas Shchelushkin () a few years before the prediction of SSW by Lifshits and Dyakonov. The charge and spin current equations obtained in Ref. Shchelushkin, are reproduced below

(3) | |||||

Here, is the spin-independent chemical potential, is the -th component of the spin-dependent chemical potential, and is the unitless spin-orbit parameter. The metallic system is described in terms of its free electron Fermi wave vector and its mean free path . is the charge current density and is the spin current density defined as a vector in the direction of the spin polarization, flowing along the direction . The first terms in Eqs. (3) and (II) are the diffusion terms, the second terms () are the side jump contribution producing SHE [Eq. (II)] and inverse SHE [Eq. (3)]. The third term in Eq. (II) is the spin swapping effect. Note that since these equations are derived within the first Born approximation (i.e. up to the second order in impurity potential only), skew scattering is neglected (see also Ref. Shchelushkin2006, ). The spin swapping term in Eq. (II) clearly converts into , which is consistent with Lifshits and Dyakonov theory lifshits_prl2009 (). A simplified version of the drift-diffusion equations, Eqs. (3)-(II), has been numerically investigated by Sadjina et al. sadjina2012 (), neglecting SHE.

A second interesting aspect of SSW is that since it comes from impurity scattering, it can be engineered by using resonant scattering on heavy impurities embedded in a light metal host as suggested previously for SHE Guo2009 (); tanaka2009 (); fert2011 (); levy2013 (). This aspect is beyond the scope of the present work, but deserves further investigations.

## Iii Tight binding model

The drift-diffusion model presented in the previous section, Eqs. (3)-(II), has been obtained within the first Born approximation, i.e. only accounting for effects proportional to the impurity density and up to the second order in impurity potential Shchelushkin (); Shchelushkin2006 (). Therefore, configurational averaging is performed and skew scattering is neglected. In this model, the ratio between SHE [second term in Eq. (II)] and (side-jump only) SSW [third term in Eq. (II)] is .

The objective of the present work is to investigate the nature of spin-orbit coupled transport (i.e. SSW, SHE and spin relaxation) over a broad range of disorder strengths and accounting for all the relevant contributions to extrinsic SHE (side-jump, skew scattering etc.). To do so, we consider a tight-binding model on which spin-orbit coupled disorder is implemented. By computing the non-equilibrium local spin density that accumulates at the edges of the sample, one can evaluate the relative magnitude of SSW and SHE, identify its dependence as a function of the disorder strength and clarify the role of spin relaxation.

The metallic system we consider is sketched in Fig. 2(a) and (b). It is composed of a ferromagnet (FM) polarized along and a normal metal (NM) with spin-orbit coupled disorder (see below). Following the discussion given in the previous section, we choose the FM polarization along to insure that the spin density injected in the normal metal does not readily undergo SHE as long as the spin polarization is conserved [see Fig. 2(a)]. Therefore, we expect SSW to take place in a region close to the interface and limited by the spin relaxation length. This SSW generates a spin accumulation at the edges of the sample whose polarization is aligned with the direction of injection ( in this example). While the injected spin accumulation is relaxed, over a distance of the order of the spin diffusion length , SHE smoothly takes over and a spin accumulation at the edges of the sample and polarized along the normal of the plane emerges. We numerically demonstrate this scenario using the tight-binding model described below.

The calculations carried out in the present work are based on the non-equilibrium Green’s function technique implemented on a single band tight-binding model kwant (). All the expectation values of the physical quantities of interest are given in real space. The whole system sketched in Fig. 2(b), i.e. the FM/NM bilayer, is connected to two non-magnetic semi-infinite leads whose role boils down to maintaining the flow of the particles throughout the system and hence promoting the non-equilibrium regime. The total Hamiltonian of the central system reads

Here the first term at the right-hand side of Eq. (III) is the spin-independent onsite energy in which , being the onsite energy constant and being a random onsite energy that introduces disorder in the system. The local disorder strength is randomly chosen such that . The second term stands for the exchange interaction between the spin of the carriers and the local magnetic momentum of site , is the exchange splitting, is the unit vector along the direction of the local magnetic moment on site . In the present case, in the FM layer and in the NM region. The operator () creates (annihilates) a particle with spin at position . The third term in the Hamiltonian corresponds to the nearest neighbor hopping energy parameterized by the hopping integral .

The SOC Hamiltonian is given by the second term in Eq. (1) and can be discretized on the square lattice we consider. Since two spatial gradients are involved ( and ), this term yields a spin-dependent next-nearest neighbor hopping contribution and can be rewritten pareek2001 ()

(6) |

where are unit vectors pointing from the initial position to the nearest neighbor and from the nearest neighbor to the next-nearest neighbor, respectively, and is the onsite energy of the nearest neighbor. Hence for a two-dimensional system, reduces to two kinds of hopping involving the disordered-onsite energiespareek2001 ()

(7) | |||

(8) |

where and is the lattice parameter. The hopping from the site to the site can either pass by or by which give opposite contributions to the spin-orbit field. The same reasoning applies for the hopping from site to site . In the present study, we choose the tight-binding parameters to be in units of the hopping energy : the transport energy , the exchange interaction between the carrier spin and the local magnetic moment is, unless stated otherwise, given by . The SOC and disorder strengths ( and ) range from ( to and to respectively).

The effects we are interested in - SSW, SHE and spin relaxation - arise from the conjunction of disorder and SOC and hence only emerge when configurational averaging is properly carried out. The advantage of the tight-binding approach is that once the calculations are converged, mechanisms such as skew-scatteringsmit_1955 (); smit_1958 () and side jumpberger_1970 () are fully accounted for. Therefore in the present work, each numerical result has been averaged over 10 configurations and convergency has been verified.

## Iv Numerical results

In this section we present the non-equilibrium calculations obtained using the Kwant code kwant (). An important criterion in the investigation of disorder-driven effects is the determination of the effective mean free path of the system, as a function of the strength of the disorder. To do so, we used the semiclassical formula for the conductance

(9) |

where is the actual conductance of the sample, is the ballistic conductance, is the length of the sample and is the mean free path. This formula indicates that as long as the mean free path is well defined, the ratio should remain constant when varying . In principle, Eq. (9) is only valid as long as localization effects are weak and when SOC is absent. The effective mean free path extracted from our numerical calculations are displayed in Fig. 3 (the conductance is shown in the inset, for reference) and exhibits no dependence as a function of the length of the sample (except for very weak disorder - blue symbols - which indicates that the transport is not in the diffusive regime). These straight lines constitute a sane signature that the regime is diffusive in this parameter space. From now on, we choose the disorder strength in the range where the mean free path in Fig. 3 shows a constant profile.

### iv.1 Crossover between spin swapping and spin Hall effects.

In order to study the crossover between SHE and SSW, we consider the structure depicted in Fig. 2(a). The current is injected from the FM layer into the NM layer along -direction. Figure 4 displays the two dimensional map of the - and -components of the spin density, and , for different strengths of the SOC unitless parameter, =0.3 and =0.6. The spatial profile of the three components of the spin density taken along a line passing by the center of the sample is shown in Fig. 5. Since the magnetization of the FM layer is aligned along the -direction, the injected current is spin polarized transversally to the direction of injection. The transverse component of the spin density simply relaxes in the NM due to SOC-driven spin relaxation [see Fig. 5, green symbols]. Interestingly, the injected spin current immediately experiences spin swapping, which results in the accumulation of the spin density along the edges of the sample, close to the FM/NM interface. This accumulation vanishes over a length of the order of the spin diffusion length. Simultaneously, as the injected spin current gets progressively depolarized through spin relaxation, a spin density accumulates at the edges of the sample due to SHE. In contrast with , survives away from the FM/NM and is maintained throughout the length of the sample. This crossover between SSW and SHE is therefore controlled by the spin relaxation length, in agreement with the scenario exposed in Section II.

It clearly appears that the injected spin current is converted into upon scattering in the normal metal, in agreement with the phenomenological prediction of Lifshits and Dyakonov lifshits_prl2009 () and with the drift-diffusion model given by Shchelushkin and Brataas Shchelushkin (). One can recover the spin density profile induced by SSW in Figs. 4(a,c) by solving the diffusive transport equations, Eqs. (3)-(II), to the lowest order in SOC. In the configuration adopted in the present work, the spin accumulation injected in NM has the form , where depends on the material parameters valet1993 () (conductivity, polarization, interfacial resistance etc.). In the presence of SOC, the magnitude acquires a dependence on and one finds that the spin accumulation at the edges is

(10) |

This solution shows that the spin relaxation plays an important role in the build-up of the spin accumulation induced by SSW. In the absence of spin relaxation, no spin current is generated and therefore SSW is inactive. But on the other hand, when spin relaxation is too strong, obviously, the spin accumulation at the edges of the sample does not extend away from the interface.

### iv.2 Dependence on the SOC strength

The relative magnitude of the spin density accumulated through SSW and SHE depends on the strength of the SOC parameter in a nonlinear manner, which is at first sight quite surprising since both effects are, in principle, proportional to the SOC strength. However, the spin relaxation is detrimental to the spin swapping since it limits the amount of spin density available for the swapping. Indeed, Fig. 6 shows the two dimensional mapping of for different strengths of SOC. The induced spin density is localized at the edges of the sample and extents over away from the interface. The spin relaxation length decreases when the SOC strength increases from () to ().

The interplay between the scattering events mentioned above in conjunction with the spin relaxation lead to the emergence of two regimes which characterize the dependence of the SSW accumulation on the SOC strength . The weak SOC regime corresponds to the enhancement of the spin swapping phenomena simply driven by the increase of the conversion efficiency with SOClifshits_prl2009 (), while the spin relaxation remains limited. For relatively larger values of SOC (), the SSW accumulation decreases in magnitude when increases (Fig. 7). The -component of the spin density varies from to for varying from to . Indeed, while the conversion efficiency increases with , the spin relaxation reduces the amount of spin current that is available for swapping. At large enough , the spin relaxation dominates and the spin swapping decreases. When increases, the spin relaxation length (the extent of the spin accumulation at the edges) decreases from for to for . It is remarkable to notice that while SSW has a non linear dependence as a function of , SHE homogeneously increases with . Indeed spin relaxation, as it depolarizes the injected spin current in NM, favors SHE.

### iv.3 Influence of the disorder

As mentioned in Section III, the disorder is a mandatory ingredient in our model to get all the effects previously discussed, a fact that elucidates the pure extrinsic origin of the SSW effect. In order to identify the impact of disorder on SHE and SSW, we numerically calculate the spin density profile for various strengths of disorder (i.e. different mean free paths). Similarly to what has been noted for the dependence of the SSW accumulation on , the disorder dependence exhibits the two regimes mentioned above. While the SOC strength controls the coupling between the spin and orbital momenta, the disorder strength controls the scattering probability off the impurities.

Figure 8 represents the spatial profile of the - and - components of the spin accumulation at the edge of the sample for different disorder strengths. In these calculations, the effective mean free path ranges from ( eV) to ( eV). Quite remarkably, while the extension of the SSW-induced spin accumulation within the normal metal decreases when increasing the disorder strength [see Figs. 8(a) and (c)], the overall magnitude of the edge spin accumulation is only weakly sensitive to [see Figs. 8(b)]. This indicates that the magnitude of the SSW effect is mostly controlled by the spin relaxation strength, while the SSW efficiency itself remains independent on the disorder. This observation is consistent with the diffusive model which states that the SSW-induced spin current is proportional to the SOC strength only [see last term in Eq. (II)], while the edge spin accumulation is controlled by the spin diffusion length [see Eq. (10)]. This behavior sharply contrasts with the dependence on the SHE-induced edge spin accumulation displayed in Fig. 8(d). Indeed, our calculations show that the magnitude of the SHE-induced spin accumulation is on contrary very sensitive to the disorder strength and almost vanishes for eV, whereas SSW survives. This is, again, consistent with the diffusive model, Eq. (II), that shows that in our model extrinsic SHE necessitates a large amount of disorder to emerge.

## V Observing spin swapping

Before concluding this study, we propose three setups for the experimental detection of the spin swapping. The first setup, displayed on Fig. 9(a), relies on direct spin injection. A spin-polarized charge current is injected along the direction from a polarizer (denoted F1) into a normal metal possessing strong SOC (red layer). Since the magnetization of the polarizer F1 is aligned along , the spin swapping generates a spin current flowing along the direction and spin-polarized along . This spin current accumulates spins (red arrows) at the interface with a second ferromagnet, F2. By sweeping the magnetization of F2 along (or by simply reversing the direction of the injected current), one should collect a magnetoresistive signal arising from the interfacial spin accumulation produced by the spin swapping. The main constraint of this setup is that the area of the ferromagnet F2 in contact with the normal metal must be at most of the order of to maximize the detection.

The second method we propose, displayed on Fig. 9(b), relies on non-local spin injection and may be simpler to fabricate. A spin-polarized charge current is injected along , from a polarizer (denoted F1) into the normal metal (red layer). A pure spin current, free of charge and spin-polarized along the magnetization direction of F1 aligned along , diffuses along (blue arrows). Through spin swapping, a spin current polarized along and flowing along is injected into a second ferromagnet F2 placed on top of the normal metal. Again, by sweeping the magnetization of F2 along or by reversing the direction of the injected current, one should collect a magnetoresistive signal arising from the spin swapping. The main constraint of this setup is that the distance between F1 and F2 must be smaller than . This setup presents some similarities with the famous spin field-effect transistor proposed by Datta and Das datta90 (), whose operation relies on coherent spin precession induced by Rashba SOC rather than spin-orbit coupled impurities.

The two previous setups present the inconvenience of being limited by the spin diffusion length of the spin-orbit coupled metal. One alternative situation is depicted in Fig. 9(c), which is a variant of the setup displayed in Fig. 9(a). This structure consists in a Hall cross where a spin current is injected from a first ferromagnet F1 into the cross and spin-orbit coupled impurities are only present in the center of the cross. For instance, if one imagines a Hall cross made of Cu, doping the center of the cross with, say, Bismuth impurities would allow for the spin swapping to take place at this location only while preventing spin relaxation in the branches of the cross. The detection of the spin swapping-induced spin current can be achieved by performing a magnetoresistance measurement on F2. Another advantage is that the magnetization direction of F1 and F2 are both in-plane.

## Vi Conclusion

We have shown that spin-orbit coupled disorder induces a strong SSW that may even exceed extrinsic SHE in metals. The crossover between these two effects is controlled by the spin relaxation of the injected spin current. While both SSW and SHE emerge through scattering on spin-orbit coupled disorder, these two effects present a noticeably different dependence as a function of both the SOC and disorder strengths. Indeed, while SHE monotonously increases with the SOC strength, SSW displays a more complex behavior due to the competition with spin relaxation. In addition, while SHE is very sensitive to the disorder strength, it turns out that the SSW efficiency is rather controlled by spin relaxation than by the disorder strength itself.

Finally, we propose three experimental setups that shall allow for the experimental detection of the spin swapping in metals possessing impurities-driven spin-orbit coupling. Materials in which extrinsic SHE dominates over the intrinsic contributions, such as heavy metal-doped light metals such Au(Pt) Guo2009 (), Au(W) Laczkowski2014 (), Cu(Ir) niimi_prl2011 (), Cu(Bi) niimi_prl2012 (), or even rare-earth doped metals tanaka2009 (), are attractive candidates for the observation of this effect as they associate strong spin Hall angle with a reasonably long spin diffusion length.

###### Acknowledgements.

A.M. acknowledges inspiring discussions with T. Valet on the physics of spin swapping and H.B.M.S. thanks S. Feki for his valuable technical support. For computer time, this research used the resources of the Supercomputing Laboratory at King Abdullah University of Science and Technology (KAUST) in Thuwal, Saudi Arabia. Y.O. acknowledges support from Grant-in-Aid for Scientific Research on Innovative Areas ”Nano Spin Conversion Science” (Grant No. 26103002).## References

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